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However, their practical implementations remain constrained by some challenges, including sluggish oxygen reduction\/evolution reaction (ORR\/OER) kinetics and insufficient electrochemical stability of conventional electrolyte systems. Halogens and halides have multiple advantages, whether it is the strong electronic modulation capability possessed by F, the modification of electrolytes by Cl and Br, or the replacement of OER by the iodine oxidation reaction (IOR), all of which can solve various pain points for high\u2010performance ZABs. Based on these advantages, the review systematically summarizes the research advancements of halogens and halides in ZABs. First, the review provides a concise overview of ZABs. Subsequently, from the perspectives of component modulation, defect engineering, interface regulation, and electrolyte modification, the review elaborates in detail the multifaceted regulatory mechanisms of fluorine, chlorine, bromine, and iodine and their compounds in enhancing catalytic activity and optimizing battery performance. Finally, the review summarizes the synergistic effects in halogen systems, outlines the remaining challenges, and offers some valuable insights for designing high\u2010efficiency ZABs, while holding significant implications for advancing sustainable renewable energy storage technologies.<\/jats:p>","DOI":"10.1002\/smll.202507843","type":"journal-article","created":{"date-parts":[[2025,10,7]],"date-time":"2025-10-07T10:35:18Z","timestamp":1759833318000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["The Dual Role of Halides in Zinc\u2013Air Batteries: From Catalytic Modulator to Electrolyte Stabilizer"],"prefix":"10.1002","volume":"21","author":[{"given":"Chengwei","family":"Liu","sequence":"first","affiliation":[{"name":"Ministry of Education Key Laboratory for Advanced Textile Composite Materials, School of Textile Science and Engineering Tiangong University  Tianjin 300387 P. R. 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