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However, the fabrication of these composites with minimal complexity and equipment requirements remains challenging. Here, we present a facile humidity\u2010triggered nonsolvent vapor\u2010induced phase separation (NVIPS) approach to fabricate 3D porous composites using a thermoplastic polyurethane solution on reduced graphene oxide\u2010modified carbon fiber felt under ambient conditions. The fabricated composites exhibit exceptional piezoresistive stability with rapid response (60\u00a0ms), a broad pressure detection range, high air permeability (358\u00a0mm s\n                    <jats:sup>\u22121<\/jats:sup>\n                    ), and outstanding X\u2010band EMI shielding (74\u00a0dB). Moreover, by integrating a neural network model, an intelligent cognition system capable of real\u2010time recognition of the object material species is constructed via robotic touch under varying pressures (accuracy\u00a0&gt;\u00a097.8%). Our bioinspired NVIPS strategy offers a versatile solution for multifunctional sensing and EMI protection through the highly flexible, breathable, and conductive porous composites.\n                  <\/jats:p>","DOI":"10.1002\/smll.202509930","type":"journal-article","created":{"date-parts":[[2026,1,12]],"date-time":"2026-01-12T15:29:30Z","timestamp":1768231770000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Humidity\u2010Triggered Spontaneous Phase Separation Enables Multifunctional 3D Porous Composites for Piezoresistive Mechanosensory and Electromagnetic Interference Shielding"],"prefix":"10.1002","volume":"22","author":[{"given":"Yige","family":"Liu","sequence":"first","affiliation":[{"name":"College of Textiles (International silk Institute) Key Laboratory of Advanced Textile Materials and Manufacturing Technology (Zhejiang Sci\u2010Tech University) Ministry of Education  Hangzhou 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