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The unsatisfactory adsorption and activation of CO\n                    <jats:sub>2<\/jats:sub>\n                    suppress electrochemical reduction over a narrow potential window. Herein, we synthesized CO\n                    <jats:sub>2<\/jats:sub>\n                    adsorption\u2010enhanced bismuth oxide nanosheets (syn\u2010Bi\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    ) using a one\u2010pot low\u2010temperature water bath method. The syn\u2010Bi\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    exhibited marked Faradic efficiency (FE\n                    <jats:sub>formate<\/jats:sub>\n                    ) over 94% in a wide potential window from \u22120.43 to \u22121.31\u00a0V versus RHE in the flow cell, and demonstrated an appreciable FE\n                    <jats:sub>formate<\/jats:sub>\n                    of 94.5% at a partial current density of 661.9\u00a0mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . The in situ spectroscopy and theoretical calculation unraveled the distinct formate production performance of the syn\u2010Bi\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    catalyst, which was contributed by its adsorption of CO\n                    <jats:sub>2<\/jats:sub>\n                    and promoting the subsequent formation of intermediates. Furthermore, coupled with the simulated solar cell with the 4 layer 3\u2010cell stacks, the solar to formate and overall solar\u2010to\u2010fuel reach 19.34% and 20.23% with over 0.21\u00a0A, respectively. This work provides insights into the practical application of electrochemical CO\n                    <jats:sub>2<\/jats:sub>\n                    reduction for formate production driven by solar energy.\n                  <\/jats:p>","DOI":"10.1002\/smll.202512691","type":"journal-article","created":{"date-parts":[[2026,1,8]],"date-time":"2026-01-08T11:36:18Z","timestamp":1767872178000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Adsorption\u2010Enhanced Bismuth Oxide Efficiently Convert CO\n                    <sub>2<\/sub>\n                    to Formate Over a Wide Potential Window"],"prefix":"10.1002","volume":"22","author":[{"given":"Dan","family":"Lei","sequence":"first","affiliation":[{"name":"International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University  Xi'an P. R. 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