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Herein, we have developed an excellent impact\u2010resistant adhesive suitable for underwater applications by hydrophobic protective B\u2500O bonds. This design enables rapid energy dissipation upon impact while the hydrophobic components protect the dynamic B\u2500O bonds from hydrolysis, ensuring reliable underwater adhesion. The resulting adhesive achieves an adhesive strength of 1.01\u00a0MPa under dry conditions and retains over 90% of its strength under water, significantly outperforming the 3\u00a0\n                    <jats:sc>m<\/jats:sc>\n                    commercial adhesive (0.49\u00a0MPa). It also exhibits an impact force attenuation efficiency of up to 83.3%; when configured into a sandwich structure, the efficiency maintains high levels of 85.9% and 87.7% under dry and water\u2010immersed conditions, respectively, with excellent structural integrity. This work provides a straightforward and effective strategy for developing high\u2010performance underwater impact\u2010resistant adhesives.\n                  <\/jats:p>","DOI":"10.1002\/smll.202514263","type":"journal-article","created":{"date-parts":[[2026,2,12]],"date-time":"2026-02-12T18:49:46Z","timestamp":1770922186000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Impact\u2010Resistant Underwater Adhesive Based on the Shear\u2010Stiffening Effect via Hydrophobic Protective B\u2500O Bonds"],"prefix":"10.1002","volume":"22","author":[{"given":"Minjie","family":"Cai","sequence":"first","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenyi","family":"Xie","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haitao","family":"Wu","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Huang","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of Advanced Polymer Materials Sichuan University  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hongle","family":"Liu","sequence":"additional","affiliation":[{"name":"EMT New Material LLC  Mianyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Wu","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering State Key Laboratory of 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