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Their reliability can be enhanced by integrating phase change materials (PCMs) to buffer thermal fluctuations and ensure stable operation, yet conventional PCMs often suffer from low thermal conductivity and poor solar capture. Herein, photosensitive Co\/C\u2010anchored reduced graphene oxide (rGO) conductive framework was fabricated via metal\u2010organic framework (MOF) pyrolysis\u2010assisted zinc volatilization strategy. This design enables the in situ formation of MOF\u2010derived uniformly dispersed cobalt nanoparticles within rGO framework. After the encapsulation of paraffin wax (PW), the resultant rGO@Co\/C\u2010PW composite PCMs demonstrate a remarkable solar\u2010thermal conversion efficiency of 92.5% under 100 mW\u00b7cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    irradiation, attributed to the synergistic interplay between the broadband absorption and non\u2010radiative relaxation of graphitic carbon and the localized surface plasmon resonance of Co nanoparticles. rGO@Co\/C\u2010PW also exhibits enhanced thermal conductivity, high phase change enthalpy, and excellent long\u2010term cycling stability, supported by regulated non\u2010isothermal phase transition kinetics via heterogeneous nucleation and spatial confinement. When integrated into a thermoelectric module, a sustained and stable power output of 8.82\u00a0mW under 100\u00a0mW\u00b7cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    is generated, capable of powering small electronic devices. This study provides valuable insights into developing next\u2010generation PCMs integrating solar\u2010thermal conversion, thermal energy storage, and thermoelectric output.\n                  <\/jats:p>","DOI":"10.1002\/smll.73606","type":"journal-article","created":{"date-parts":[[2026,5,5]],"date-time":"2026-05-05T08:46:28Z","timestamp":1777970788000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Modulating Photons and Phonons in Graphene\u2010Based Phase Change Materials for Solar\u2010Thermal\u2010Electrical Generation"],"prefix":"10.1002","volume":"22","author":[{"given":"Shuaihua","family":"Yuan","sequence":"first","affiliation":[{"name":"School of Materials Design and Engineering Beijing Institute of Fashion Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiaying","family":"Zhu","sequence":"additional","affiliation":[{"name":"School of Engineering The University 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