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Although the deliberate incorporation of chiral molecules into local coordination environments has imparted remarkably tailored chiroptical and spintronic responses in synthetic systems, such as organic frameworks and hybrid organic\u2010inorganic perovskites, translating such chiral control into the well\u2010explored 2D layered materials (e.g., graphene and transition metal dichalcogenides) faces substantial hurdles, including precise nanostructure fabrication, molecular assembly, subtle chiral coupling, and reliable electronic and optical characterization. This review systematically outlines up\u2010to\u2010date feasible strategies for chiral engineering in 2D layered materials to leverage their functional landscape and unlock the emergent chiral properties. It begins with intrinsic and extrinsic engineering approaches, highlighting the underlying design principles and the resulting novel physical and chemical behaviors. We further discuss potential extensions of these chirality\u2010engineering approaches and explore future promising opportunities that harness rationally tailored chiral functionalities in 2D systems for next\u2010generation optoelectronics, spintronics, and quantum information science.<\/jats:p>","DOI":"10.1002\/smll.73856","type":"journal-article","created":{"date-parts":[[2026,5,30]],"date-time":"2026-05-30T10:46:16Z","timestamp":1780137976000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Chirality Engineering and Properties in Two\u2010Dimensional Layered Materials"],"prefix":"10.1002","volume":"22","author":[{"given":"Junwei","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Synergistic Chem\u2010Bio Synthesis School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai China"},{"name":"Key Laboratory of Intelligent Creation for Extreme Energy 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