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Although the polyvinylidene fluoride (PVDF) and its derivatives have achieved great progresses in OTENGs, the unsatisfactory electronegativity induced by their low polar\n                    <jats:italic>\u03b2<\/jats:italic>\n                    \u2010phase remains a huge challenge for a high\u2010performance electricity output. Herein, the self\u2010assembled 1,3,5\u2010Tris\u2010(4\u2010aminophenyl) benzene (TAPB)\u20101,2,4,5\u2010tetracyanobenzene (TCNB) charge\u2010transfer (CT) cocrystals with a considerable dielectric constant of 10.2 were purposefully introduced into PVDF\u2010co\u2010hexafluoropropylene (PVDF\u2010HFP) matrix via a spin\u2010coating process to enhance its electronegativity. By sandwiching the composite film between Ag electrodes on the polyethylene terephthalate (PET) substrates, OTENGs with remarkable mechanical durability and reversible deformability were successfully prepared. The introduced TAPB\u2010TCNB cocrystal could significantly enhance the dielectric response and polar\n                    <jats:italic>\u03b2<\/jats:italic>\n                    \u2010phase of PVDF\u2010HFP film, which is beneficial for a fivefold voltage output of 90\u00a0V compared to pure PVDF\u2010HFP OTENGs, and sensitivity of 2.926\u00a0V\u00a0N\n                    <jats:sup>\u22121<\/jats:sup>\n                    with the outstanding stability over 5000 cycles under the pressure of 50\u00a0N. Furthermore, the proposed devices hold strong potential for self\u2010powered wearable sensing applications, including human motion monitoring, gait analysis, and Morse\u2010code\u2010based communication.\n                  <\/jats:p>","DOI":"10.1002\/smll.74232","type":"journal-article","created":{"date-parts":[[2026,6,16]],"date-time":"2026-06-16T17:16:47Z","timestamp":1781630207000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Organic Charge\u2010Transfer Dielectric Cocrystals for Flexible Triboelectric Nanogenerators and Wearable Application"],"prefix":"10.1002","volume":"22","author":[{"given":"Dan","family":"Chen","sequence":"first","affiliation":[{"name":"China National Textile and Apparel Council Key Laboratory for Silk Functional Materials and Technology National Engineering Laboratory for Modern Silk College of Textile and Clothing Engineering Soochow University  Suzhou Jiangsu 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Engineering Soochow University  Suzhou Jiangsu China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,6,16]]},"reference":[{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.pmatsci.2023.101184"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202307918"},{"key":"e_1_2_7_4_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202403791"},{"key":"e_1_2_7_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2024.110253"},{"key":"e_1_2_7_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010019\u201009464\u20108"},{"key":"e_1_2_7_7_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.physrep.2018.11.001"},{"key":"e_1_2_7_8_1","first-page":"1641","article-title":"Triboelectric Nanogenerator Array as a Probe for In Situ Dynamic Mapping of Interface Charge Transfer at a Liquid\u2010Solid Contacting","volume":"17","author":"Zhang J.","year":"2023","journal-title":"ACS 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