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Here, we overcome this barrier by introducing lithium sulfonate\u2010functionalized mesoporous silica (M\u2010SiO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010SO\n                    <jats:sub>3<\/jats:sub>\n                    Li) as a multifunctional filler. Unlike conventional fillers that impede ion transport, M\u2010SiO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010SO\n                    <jats:sub>3<\/jats:sub>\n                    Li simultaneously induces shear thickening and enhances conductivity. At 15\u00a0wt.% loading, the electrolyte achieves a remarkable ionic conductivity of 10.73 mS cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    , higher than that of filler\u2010free traditional electrolytes (TE), by anchoring anions via the \u2010SO\n                    <jats:sub>3<\/jats:sub>\n                    Li groups to increase the Li\n                    <jats:sup>+<\/jats:sup>\n                    transference number. This synergy enables exceptional battery performance: Li||LFP cells demonstrate 97.0% capacity retention after 500 cycles, and LFP||Gr pouch full cells maintain 83.8% capacity after 200 cycles at 0.5 C. In impact tests, the robustness of this design is evident as the M\u2010SiO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010SO\n                    <jats:sub>3<\/jats:sub>\n                    Li\u2010based pouch cell withstands hammer drops that cause immediate failure in standard TE cells. Thus, this design strategy overcomes the performance trade\u2010off, integrating high conductivity, long cycling life, and impact resistance, and provides a pathway for application across the liquid\u2010based electrolyte family.\n                  <\/jats:p>","DOI":"10.1002\/smll.74488","type":"journal-article","created":{"date-parts":[[2026,7,10]],"date-time":"2026-07-10T08:47:31Z","timestamp":1783673251000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Impact\u2010Tolerant Batteries Enabled by High\u2010Conductivity Shear Thickening Electrolytes"],"prefix":"10.1002","volume":"22","author":[{"given":"Quan","family":"Liu","sequence":"first","affiliation":[{"name":"Department of Modern Mechanics CAS Key Laboratory of Mechanical Behavior and Design of Materials University of Science and Technology of China  Hefei Anhui P. R. 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