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But they often exhibit a considerable increase in thermal conductivity at high temperatures, which could lead to a serious catastrophe in actual applications. Meanwhile, simultaneously achieving high compressive strength and superelasticity for porous ceramic structures remains a challenge. Herein, we propose one kind of novel lamellar\u2010structured ceramic nanofiber aerogel, where the deliberately tailored ZrP\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>7<\/jats:sub>\n                    and AlPO\n                    <jats:sub>4<\/jats:sub>\n                    are used as functional constituents and form inter\u2010nanofiber bonding. By this strategy, the prepared aerogels achieve the synergistic integration of three core properties: a 90% fully recoverable strain that far outperforms the vast majority of reported ceramic aerogels, an ultrahigh compressive strength of 1097 kPa at 90% strain, and a thermal conductivity as low as 0.089 W\u00b7m\n                    <jats:sup>\u2212<\/jats:sup>\n                    <jats:sup>1<\/jats:sup>\n                    \u00b7K\n                    <jats:sup>\u2212<\/jats:sup>\n                    <jats:sup>1<\/jats:sup>\n                    at 1000\u00b0C. The experimental and theoretical analysis results show that the unique layered structure with robust crosslinking design can effectively improve the structural stability and compressive strength, while phosphate compounds can reduce high\u2010temperature radiative heat transfer. This work provides a new perspective for collaborative design of mechanical and thermal properties of advanced ceramic aerogels.\n                  <\/jats:p>","DOI":"10.1002\/smll.75392","type":"journal-article","created":{"date-parts":[[2026,8,21]],"date-time":"2026-08-21T09:41:26Z","timestamp":1787305286000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Ultrastrong yet Superelastic Lamellar Ceramic Aerogels Achieved through Inter\u2010Nanofiber Bonding for High\u2010Temperature Thermal Insulation"],"prefix":"10.1002","author":[{"given":"Lei","family":"Wen","sequence":"first","affiliation":[{"name":"National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of Technology  Harbin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yichen","family":"Zhou","sequence":"additional","affiliation":[{"name":"National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of Technology  Harbin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yushun","family":"Zhao","sequence":"additional","affiliation":[{"name":"National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of Technology  Harbin China"},{"name":"School of Astronautics Harbin Institute of Technology  Harbin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenxi","family":"Zhao","sequence":"additional","affiliation":[{"name":"National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of Technology  Harbin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaodong","family":"Sun","sequence":"additional","affiliation":[{"name":"School of Astronautics Harbin Institute of Technology  Harbin 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