{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T11:15:50Z","timestamp":1788347750293,"version":"build-2803163510"},"reference-count":50,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T00:00:00Z","timestamp":1788307200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T00:00:00Z","timestamp":1788307200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22075330"],"award-info":[{"award-number":["22075330"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22379029"],"award-info":[{"award-number":["22379029"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["U24A20569"],"award-info":[{"award-number":["U24A20569"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52271204"],"award-info":[{"award-number":["52271204"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    The anode\u2010cathode crosstalk, driven by bilateral OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    and polyhalide shuttling, forms an underestimated vicious cycle that critically degrades the capacity of aqueous Zn halogen batteries (AZHBs). In this cycle, anode corrosion produces OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    , whose migration exacerbates cathode decay and polyhalide shuttling, which in turn leads to corrosion and increased OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    production at the anode. To break such a self\u2010amplifying degradation cycle, we develop a Janus separator functionalized with a porous ZIF\u20108 material encapsulated with benzotriazole (BTA) inhibitor. This layer is placed on the cathode side, where its ordered channels physically confine polyhalide shuttling, preventing corrosive species from reaching the Zn anode. Concurrently, BTA can be sustainably released from ZIF\u20108 framework, forming a stable solid\u2010electrolyte interphase on Zn anode to isolate water\u2010involved side reactions. By blocking polyhalide crossover and eliminating water\u2010induced OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    supply, this Janus design severs the OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    \u2010driven vicious cycle at its source, without requiring additional electrolyte additives or complex anode modifications. Consequently, Zn||I\n                    <jats:sub>2<\/jats:sub>\n                    and Zn||TBABr\n                    <jats:sub>3<\/jats:sub>\n                    batteries incorporating the Janus separator achieve a three\u2010fold extension in cycle life compared to batteries with a conventional separator, confirming that interrupting OH\n                    <jats:sup>\u2212<\/jats:sup>\n                    migration effectively halts the autocatalytic degradation pathway. Breaking this previously underestimated degradation mechanism provides a new route toward high\u2010stability AZHBs.\n                  <\/jats:p>","DOI":"10.1002\/smll.75479","type":"journal-article","created":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T10:40:51Z","timestamp":1788345651000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Breaking the Underestimated Vicious Cycle of OH\n                    <sup>\u2212<\/sup>\n                    Migration via a Janus Separator in Aqueous Zn\u2013Halogen Batteries"],"prefix":"10.1002","author":[{"given":"Guoli","family":"Liao","sequence":"first","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yueliang","family":"Chen","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhaoyu","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaojia","family":"Lan","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yufei","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2779-2557","authenticated-orcid":false,"given":"Minghui","family":"Ye","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang 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