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However, their fundamental design principles, entropy\u2010driven mechanisms, and structure\u2013performance relationships remain poorly understood, limiting their rational development. This review provides a timely update on the recent progress of HE LRCs, offering an overview of the entropy concept and HE effect, alongside a comprehensive summary of their crystal structures, compositions, and properties. Additionally, it summarizes emerging design strategies, including multi\u2010element doping and entropy\u2010assisted surface engineering, and highlights the growing role of machine learning in accelerating the design of HE LRCs. Finally, the challenges and future development trends of HE LRCs are discussed, emphasizing the need for precise control of local chemical environments and deeper mechanistic insights. 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