{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T11:11:19Z","timestamp":1790161879134,"version":"4.1.0"},"reference-count":44,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T00:00:00Z","timestamp":1790121600000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T00:00:00Z","timestamp":1790121600000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52372083"],"award-info":[{"award-number":["52372083"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52125202"],"award-info":[{"award-number":["52125202"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    High sulfur loading is essential for the practical application of lithium\u2013sulfur (Li\u2013S) batteries but is limited by severe polysulfide shuttling, large electrode volume changes, and sluggish Li\n                    <jats:sup>+<\/jats:sup>\n                    transport. Herein, a dual\u2010crosslinked binder (DCB) is constructed through hydrogen\u2010bonding and ionic\u2010pair interactions between quaternized soy protein isolate (QSPI) and poly (acrylic acid)\u2010based LA133. The 3D crosslinked network enhances electrode mechanical integrity and adhesion, effectively alleviating structural degradation and volume variation during cycling. Meanwhile, abundant polar functional groups provide continuous Li\n                    <jats:sup>+<\/jats:sup>\n                    coordination sites, and theoretical calculations reveal a hopping\u2010mediated Li\n                    <jats:sup>+<\/jats:sup>\n                    transport pathway between adjacent coordination sites, thereby promoting polysulfide conversion. As a result, the DCB simultaneously improves electrode stability and reaction kinetics. A 1.1 Ah Li\u2013S pouch cell employing the DCB achieves a high energy density of 348\u00a0Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    and stable cycling over 60 cycles under practical conditions with a low electrolyte\/sulfur ratio of 4\u00a0\u00b5L mg\n                    <jats:sub>s<\/jats:sub>\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a low N\/P ratio of 1.5. This work offers an effective dual\u2010crosslinking strategy for regulating Li\n                    <jats:sup>+<\/jats:sup>\n                    transport and enhancing electrode stability toward practical high\u2010sulfur\u2010loading Li\u2013S batteries.\n                  <\/jats:p>","DOI":"10.1002\/smll.75845","type":"journal-article","created":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T10:27:14Z","timestamp":1790159234000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Dual\u2010Crosslinked Aqueous Binder for High Sulfur Loading Lithium\u2013Sulfur Batteries"],"prefix":"10.1002","author":[{"given":"Guobang","family":"Zhang","sequence":"first","affiliation":[{"name":"Key Laboratory for Soft Chemistry and Functional Materials of Ministry of Education Nanjing University of Science and Technology  Nanjing 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