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Monolithic integration, though ultimately desirable, is rarely tractable at early stages of material development. Progress is therefore often assessed through idealized simulations that overlook system\u2010level constraints and non\u2010idealities such as device variability, mixed\u2010signal conversions, peripheral circuit noise, and energy overhead, yielding projections that can mislead. Here we present a heterogeneously integrated platform as a necessary stepping\u2010stone toward scalable molecular\u2010silicon hardware\u2014a 64 \u00d7 64 molecular crossbar coupled with custom Si\u2010circuitry in which every interface and signal pathway is explicitly defined and directly measured, yielding a realistic map of the design space for further scale\u2010up. We demonstrate a one\u2010step vector\u2013matrix multiplication with &gt; 12\u2010bit precision, \u223c73\u00a0dB signal\u2010to\u2010noise ratio, \u223c80\u2010ns write speeds, and high write accuracy across 10\u00a0000 programming cycles without correction loops, a substantial advance over the state of the art in dot\u2010product engines. Using this platform, we execute workloads spanning signal and image processing, biomarker detection and tracking, and cryptographic operations. This work establishes the foundation on which subsequent scale\u2010up strategies, including monolithic molecular\u2013silicon integration, can be designed and assessed.<\/jats:p>","DOI":"10.1002\/smll.75874","type":"journal-article","created":{"date-parts":[[2026,10,1]],"date-time":"2026-10-01T04:29:54Z","timestamp":1790828994000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Heterogeneous Molecular\u2010Silicon Integration for Precision Neuromorphic Computing"],"prefix":"10.1002","author":[{"given":"Jitthu","family":"Joseph","sequence":"first","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-5319-6390","authenticated-orcid":false,"given":"Lohit","family":"T","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0005-9760-4904","authenticated-orcid":false,"given":"Harivignesh","family":"S","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6907-7124","authenticated-orcid":false,"given":"Deepak","family":"Sharma","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pallavi","family":"Gaur","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0005-2310-7913","authenticated-orcid":false,"given":"Nivedita","family":"Singh","sequence":"additional","affiliation":[{"name":"Centre for Neuroscience Indian Institute of Science (IISc) Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2103-1653","authenticated-orcid":false,"given":"Deepak","family":"Nair","sequence":"additional","affiliation":[{"name":"Centre for Neuroscience Indian Institute of Science (IISc) Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4364-1767","authenticated-orcid":false,"given":"Navakanta","family":"Bhat","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5104-5757","authenticated-orcid":false,"given":"Sreetosh","family":"Goswami","sequence":"additional","affiliation":[{"name":"Centre for Nano science and Engineering CeNSE Indian Institute of Science (IISc)  Bangalore India"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,30]]},"reference":[{"issue":"9","key":"e_1_2_13_2_1","doi-asserted-by":"crossref","first-page":"752","DOI":"10.1038\/s41928-025-01432-z","article-title":"Neuromorphic Pathways for Transforming AI Hardware","volume":"8","author":"Bhat N.","year":"2025","journal-title":"Nature Electronics"},{"issue":"11","key":"e_1_2_13_3_1","doi-asserted-by":"crossref","first-page":"1475","DOI":"10.1038\/s41563-024-01820-4","article-title":"Potential and Challenges of Computing with Molecular Materials","volume":"23","author":"Williams R. 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