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However, practical commercialization remains impeded by inherent bottlenecks, including sluggish sulfur redox kinetics, metal dendrite growth, and the polysulfide shuttle effect. Single\u2010atom catalysts (SACs) have emerged as a frontier solution, offering maximized atomic utilization, tunable coordination environments, and exceptional electrocatalytic activity. This review systematically summarizes recent advances in SAC\u2010enabled M\u2010S batteries. We first delineate the fundamental electrochemistry of diverse M\u2010S systems, establishing a foundation for the rational design principles and state\u2010of\u2010the\u2010art synthetic methodologies of SACs. Particular emphasis is placed on unraveling intrinsic catalytic mechanisms, highlighting the critical role of d\u2013p orbital hybridization between single\u2010atom metal centers and sulfur intermediates in lowering activation barriers and modulating bidirectional redox kinetics. Building on these mechanistic insights, we critically evaluate SAC applications across a broad spectrum\u2014from conventional Li\u2010S to emerging beyond\u2010lithium systems, including Na\u2010S, Al\u2010S, K\u2010S, Zn\u2010S, and Mg\u2010S batteries. Finally, we provide perspectives on current challenges and future directions to guide rational SAC design for high\u2010energy\u2010density, long\u2010lifespan M\u2010S electrochemistry.<\/jats:p>","DOI":"10.1002\/smll.75895","type":"journal-article","created":{"date-parts":[[2026,9,25]],"date-time":"2026-09-25T10:28:58Z","timestamp":1790332138000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Recent Progress of Single\u2010Atom Catalysts for High\u2010Performance Metal\u2010Sulfur Batteries"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0008-1456-7506","authenticated-orcid":false,"given":"Yuchen","family":"Wang","sequence":"first","affiliation":[{"name":"Ministry of Education Key Laboratory for the Green Preparation and Application of Functional Materials School of New Energy and Electrical Engineering Hubei University  Wuhan China"},{"name":"Manchester Metropolitan Joint Institute Hubei 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