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Here, high\u2010field torque magnetometry measurements are performed, revealing a previously unrecognized anisotropic spin response that reflects interaction terms beyond the standard XY or XXZ models. In combination with relativistic density functional theory calculations and magnetic force response theory, an effective low\u2010energy spin Hamiltonian is constructed, elucidating not only the observed anomalous magnetic behavior but also other recent experiments. Remarkably, the magnetic dipole interaction and the associated spin\u2010flop transition play a crucial role in driving the deviation from two\u2010dimensional spin alignment, providing direct insight into the underlying anisotropic energy hierarchy. The generalized Hamiltonian can serve as the important fundamental ground for future study, and our approach adopted here will hopefully be relevant to many other related material systems.<\/jats:p>","DOI":"10.1002\/smll.75903","type":"journal-article","created":{"date-parts":[[2026,9,26]],"date-time":"2026-09-26T10:18:09Z","timestamp":1790417889000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Crucial Role of Magnetic Dipole and Anomalous Field Dependence in NiPS\n                    <sub>3<\/sub>"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-4861-1666","authenticated-orcid":false,"given":"Do Hoon","family":"Kiem","sequence":"first","affiliation":[{"name":"Department of Physics Korea Advanced Institute of Science and Technology (KAIST)  Daejeon Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2111-4846","authenticated-orcid":false,"given":"Muhammad","family":"Nauman","sequence":"additional","affiliation":[{"name":"Department of Physics Prairie View A&amp;M University  Prairie View Texas USA"},{"name":"Institute of Science and Technology Austria (ISTA)  Klosterneuburg Austria"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6877-7049","authenticated-orcid":false,"given":"Joonyoung","family":"Choi","sequence":"additional","affiliation":[{"name":"Department of Physics Kyungpook National University  Daegu Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"David","family":"Graf","sequence":"additional","affiliation":[{"name":"National High Magnetic Field Laboratory  Tallahassee Florida USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Junghyun","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Physics and Astronomy Seoul National University  Seoul Republic of Korea"},{"name":"Center for Quantum Materials Seoul National University  Seoul Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0747-5389","authenticated-orcid":false,"given":"Heejun","family":"Yang","sequence":"additional","affiliation":[{"name":"Department of Physics and Astronomy Seoul National University  Seoul Republic of Korea"},{"name":"Center for Quantum Materials Seoul National University  Seoul Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3930-4226","authenticated-orcid":false,"given":"Je\u2010Geun","family":"Park","sequence":"additional","affiliation":[{"name":"Department of Physics and Astronomy Seoul National University  Seoul Republic of Korea"},{"name":"Center for Quantum Materials Seoul National University  Seoul Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8030-583X","authenticated-orcid":false,"given":"Younjung","family":"Jo","sequence":"additional","affiliation":[{"name":"Department of Physics Kyungpook National University  Daegu Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8089-7991","authenticated-orcid":false,"given":"Myung Joon","family":"Han","sequence":"additional","affiliation":[{"name":"Department of Physics Korea Advanced Institute of Science and Technology (KAIST)  Daejeon Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,26]]},"reference":[{"issue":"7729","key":"e_1_2_8_2_1","doi-asserted-by":"crossref","first-page":"47","DOI":"10.1038\/s41586-018-0631-z","article-title":"Magnetism in Two\u2010Dimensional van der Waals Materials","volume":"563","author":"Burch K. 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