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However, the radially divergent arrangement of particles on cylindrical current collectors creates an inherently porous active layer, allowing unconstrained binder swelling and subsequent particle detachment, which causes irreversible capacity loss. Here, we report an adhesive gel polymer electrolyte (AGPE) formed by the in situ polymerization of 2\u2010perfluorohexyl ethyl acrylate (TFOA) and triethylene glycol diacrylate (TEGDA), in which precursor infiltration into the porous active layer and interfacial anchoring mediated by perfluorinated dangling chains help preserve interparticle adhesion, while the crosslinked TEGDA network provides dimensional stability. The resulting AGPE\u2010based FLIBs deliver stable cycling over 800 cycles and exhibit improved structural stability under diverse aging conditions, retaining 87.8% of their initial capacity after 500 days of storage at 25\u00b0C and over 90% after 14 days of thermal aging at 60\u00b0C. This strategy provides a molecular approach for stabilizing high\u2010curvature fiber electrodes, thereby broadening the applicability of fiber\u2010based energy\u2010storage technologies in wearable electronics.<\/jats:p>","DOI":"10.1002\/smll.75913","type":"journal-article","created":{"date-parts":[[2026,9,22]],"date-time":"2026-09-22T14:50:09Z","timestamp":1790088609000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["In Situ\u2010Formed Adhesive Gel Polymer Electrolyte for Stabilizing High\u2010Curvature Interfaces in Fiber Lithium\u2010Ion Batteries"],"prefix":"10.1002","author":[{"given":"Jiahe","family":"Qu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science, and Institute of Fiber Materials and Devices Fudan University  Shanghai 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