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The ability to control exchange\u2010coupling within these systems is therefore highly desirable. Here, we use an atomically sharp scanning tunneling microscope probe to vertically manipulate a 2D Mott insulating honeycomb\u2010kagome metal\u2010organic framework (MOF) featuring Kondo\u2010screened local magnetic moments on Ag(111). We show that by controlling the adsorption height of the MOF, we can also controllably and reversibly change the strength of Kondo coupling between the MOF's local spins and the substrate's conduction electrons. This mechanical control of Kondo coupling could be extended to other forms of interlayer exchange coupling, potentially allowing for atomic\u2010scale design or control of spintronics\u00a0technologies.<\/jats:p>","DOI":"10.1002\/smll.75928","type":"journal-article","created":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T07:44:36Z","timestamp":1791186276000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Atomic\u2010Scale Control of Substrate\u2010Spin Coupling Via Vertical Manipulation of a 2D Metal\u2010Organic Framework"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5157-7737","authenticated-orcid":false,"given":"Benjamin","family":"Lowe","sequence":"first","affiliation":[{"name":"Institute of Physics of the Czech Academy of Sciences Prague Czech Republic"},{"name":"School of Physics and Astronomy Monash University Clayton Victoria Australia"},{"name":"ARC Centre of Excellence in 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