{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T13:02:45Z","timestamp":1790686965939,"version":"4.1.0"},"reference-count":53,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100004607","name":"Natural Science Foundation of Guangxi Province","doi-asserted-by":"publisher","award":["2025GXNSFBA069296"],"award-info":[{"award-number":["2025GXNSFBA069296"]}],"id":[{"id":"10.13039\/501100004607","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"abstract":"ABSTRACT<\/jats:title>\n \n Exposing LiCoO\n 2<\/jats:sub>\n (LCO) to voltages over 4.35 V induces both irreversible H1\u20103\/O1 phase transformation and severe interfacial reactivity, whose synergistic effects cause substantial capacity loss. Herein, an ingenious surface reconstruction and bulk doping of LCO are proposed to overcome the above bottlenecks via selenium disulfide (SeS\n 2<\/jats:sub>\n ) treatment. In detail, the substitution of O\u2010sites by Se stabilizes the lattice oxygen of LCO, alleviating harmful phase transitions. Furthermore, the formation of a stable heterojunction between the Li\n 2<\/jats:sub>\n SO\n 3<\/jats:sub>\n \/Li\n 2<\/jats:sub>\n SO\n 4<\/jats:sub>\n \/Li\n 2<\/jats:sub>\n SeO\n 4<\/jats:sub>\n composite coating and LCO grains contributes to the suppression of interfacial side reactions and provides a mechanical cushioning effect that alleviates anisotropic lattice stress. Meanwhile, the mixed coating can also provide Li to ensure continuous Li\n +<\/jats:sup>\n supplement, facilitating Li\n +<\/jats:sup>\n diffusion. More importantly, an inorganic\u2010rich cathode\u2010electrolyte interphase (CEI) layer is generated, further improving the bulk structural robustness and interfacial charge transport. Ultimately, the SeS\n 2<\/jats:sub>\n \u2010LCO exhibits a superior cyclability under 4.6 V high\u2010voltage conditions, achieving 80.6% capacity retention at 1 C for LCO\/Li half cells after 400 cycles compared with P\u2010LCO of 37.8%. Our work introduces a bulk\u2010surface synergistic modification approach to stabilize the LCO crystal structure, which can be extended to more sophisticated coating and multiple elements doping for constructing better high\u2010voltage LCO batteries.\n <\/jats:p>","DOI":"10.1002\/smll.76053","type":"journal-article","created":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T12:46:31Z","timestamp":1790685991000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Simultaneous Bulk Doping and Surface reconstruction Engineering by SeS\n 2<\/sub>\n Treatment Enable Stable High\u2010Voltage Performance of LiCoO\n 2<\/sub>\n at 4.6 V"],"prefix":"10.1002","author":[{"given":"Zhengyi","family":"Zhong","sequence":"first","affiliation":[{"name":"State Key Laboratory of Featured Metal Materials and Life\u2010cycle Safety for Composite Structures MOE Key Laboratory of New Processing Technology for Nonferrous Metals and 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