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Although MgH\n                    <jats:sub>2<\/jats:sub>\n                    possesses high hydrogen capacity and favorable safety characteristics, its practical application is limited by thermodynamic stability, sluggish kinetics, and poor cycling durability. Carbon materials provide multifunctional regulation through structural confinement, improved transport properties, interfacial electronic modulation, and defect engineering, enabling simultaneous optimization of hydrogen sorption kinetics, thermodynamics, and cycling stability. Recent progress in carbon materials with different dimensional structures and their synergistic coupling with metal catalysts is discussed, with emphasis on the underlying mechanisms, performance regulation, and future development challenges. These carbon\u2010based coupling strategies provide promising opportunities for developing high\u2010performance MgH\n                    <jats:sub>2<\/jats:sub>\n                    \u2010based hydrogen storage systems for fuel\u2010cell vehicles, renewable energy storage, and portable power applications.\n                  <\/jats:p>","DOI":"10.1002\/smll.76061","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T10:38:25Z","timestamp":1791369505000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Carbon\u2010Based Materials Enhancing Hydrogen Storage Performance of Magnesium Hydride: Mechanisms, Multidimensional Performance Regulation and Future Perspectives"],"prefix":"10.1002","author":[{"given":"Shuaishuai","family":"Cao","sequence":"first","affiliation":[{"name":"Institute of Science and Technology for New Energy Xi'an Technological University  Xi'an People's Republic of 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