{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T13:52:48Z","timestamp":1791121968097,"version":"4.1.0"},"reference-count":54,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52272195"],"award-info":[{"award-number":["52272195"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52372187"],"award-info":[{"award-number":["52372187"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["buctrc202503"],"award-info":[{"award-number":["buctrc202503"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["JZ2024HGTG0291"],"award-info":[{"award-number":["JZ2024HGTG0291"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["PA2025GDSK0054"],"award-info":[{"award-number":["PA2025GDSK0054"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Sodium metal batteries are limited by uncontrolled Na nucleation and nonuniform deposition, which originate from insufficient interfacial sodiophilicity and heterogeneous ion\/electric\u2010field transport. Herein, we design a flexible lotus\u2010root\u2010like hierarchical porous carbon nanofiber framework embedded with ultrafine vanadium nitride (VN) nanoparticles (VN@HPCNF) is developed to synchronously coordinate these two processes through synergistic electronic\u2010structure and structural engineering. Density functional theory calculations reveal that the electronic structure of VN creates intrinsically sodiophilic sites, where electron\u2010rich N atoms initiate Na adsorption and V centers stabilize Na through Na\u20103s\/V\u20103d orbital hybridization, thereby lowering the nucleation barrier. Meanwhile, COMSOL simulations reveal that the interconnected porous architecture simultaneously homogenizes the electric\u2010field distribution and Na\n                    <jats:sup>+<\/jats:sup>\n                    flux, alleviates localized current\u2010density accumulation, and guides confined and homogeneous Na deposition. The synergistic regulation of atomic\u2010scale electronic interactions and structural\u2010scale ion\/electric\u2010field transport enables dendrite\u2010free Na growth. Consequently, VN@HPCNF exhibits stable cycling over 1000\u00a0h at 2\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , a low plating\/stripping overpotential of \u224816\u00a0mV, and a high Coulombic efficiency (CE) of 99.86% at 4\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . This work identifies electronic\u2010structure\u2010induced sodiophilicity as a decisive descriptor for regulating Na deposition, providing a mechanistic design principle for stable alkali\u2010metal anodes.\n                  <\/jats:p>","DOI":"10.1002\/smll.76108","type":"journal-article","created":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T13:16:17Z","timestamp":1791119777000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Electronic\u2010Structure Engineering Coordinates Na Nucleation Thermodynamics and Deposition Kinetics for Stable Sodium Metal Batteries"],"prefix":"10.1002","author":[{"given":"Meiqi","family":"Mou","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Engineering Research Center of Advanced Composite Materials Design &amp; Application of Anhui Province Hefei University of Technology  Hefei People's Republic of 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Composite Materials Design &amp; Application of Anhui Province Hefei University of Technology  Hefei People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-2618-9108","authenticated-orcid":false,"given":"Yulei","family":"Li","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Engineering Research Center of Advanced Composite Materials Design &amp; Application of Anhui Province Hefei University of Technology  Hefei People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhongnan","family":"Cao","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Engineering Research Center of Advanced Composite Materials Design &amp; Application of Anhui Province Hefei University of Technology  Hefei People's Republic of 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