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Herein, we report an asymmetric heterostructured breathable Janus nanofibrous membrane (AHB\u2010JNM) fabricated by in situ layered electrospinning for deep learning\u2010assisted wearable sensing. The membrane combines a compact, low\u2010surface\u2010energy thermoplastic polyurethane\/polydimethylsiloxane (TPU\/PDMS) fibrous layer for dry skin contact with a porous, hydrophilic thermoplastic polyurethane\/polyethylene glycol (TPU\/PEG) fibrous layer for moisture transport and conductive network support. This asymmetric architecture promotes directional liquid transport, suppresses reverse liquid penetration, and preserves interconnected channels for air and water\u2010vapor transport. After printing a hybrid multiwalled carbon nanotube\/silver nanowire (MWCNT\/AgNW) conductive network onto the TPU\/PEG layer, the sensor achieves a gauge factor of 121.29, a strain range up to 200%, a rapid response time of 81.2\u00a0ms, and stable sensing over 10\u00a0000 loading\u2013unloading cycles. The membrane also provides cooling and warming effects of 1.4\u00b0C and 4.3\u00b0C, respectively. Combined with a deep learning algorithm, the sensor achieves 98% accuracy in Morse code recognition. These results demonstrate a structurally programmed strategy for integrating moisture regulation, thermal management, and stable electromechanical sensing in skin\u2010interfaced wearable systems.<\/jats:p>","DOI":"10.1002\/smll.76150","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T11:11:02Z","timestamp":1791371462000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Asymmetric Heterostructured Breathable Janus Nanofibrous Membranes for Deep Learning\u2010Assisted Wearable Sensing"],"prefix":"10.1002","author":[{"given":"Xuanjie","family":"Zong","sequence":"first","affiliation":[{"name":"School of Mechanical Engineering Key Laboratory of High Efficiency and Clean Mechanical Manufacture of Ministry of Education Shandong University  Jinan Shandong People's Republic of China"},{"name":"National Demonstration Center For Experimental Mechanical Engineering Education Shandong University  Jinan Shandong People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8397-5043","authenticated-orcid":false,"given":"Chengpeng","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Mechanical Engineering Key Laboratory of High Efficiency and Clean Mechanical Manufacture of Ministry of Education Shandong University  Jinan Shandong People's Republic of China"},{"name":"National Demonstration Center For Experimental Mechanical Engineering Education Shandong University  Jinan Shandong People's Republic of China"},{"name":"State Key Laboratory of Advanced Equipment and Technology for Metal Forming Shandong University  Jinan People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qikai","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Mechanical Engineering Key Laboratory of High Efficiency and Clean Mechanical Manufacture of Ministry of Education Shandong University  Jinan Shandong People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-5235-3143","authenticated-orcid":false,"given":"Nianqiang","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Mechanical Engineering Key Laboratory of High Efficiency and Clean Mechanical Manufacture of Ministry of Education Shandong University  Jinan Shandong People's Republic of China"},{"name":"National Demonstration Center For Experimental Mechanical Engineering Education Shandong University  Jinan Shandong People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Leiqiang","family":"Han","sequence":"additional","affiliation":[{"name":"Department of Clinical Pharmacy Cheeloo College of Medicine The Second Hospital Shandong University  Jinan People's Republic of 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