{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T13:49:11Z","timestamp":1791985751977,"version":"4.4.0"},"reference-count":71,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T00:00:00Z","timestamp":1791936000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T00:00:00Z","timestamp":1791936000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2022YFD70050101"],"award-info":[{"award-number":["2022YFD70050101"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>Compartmentalized dynamic supramolecular structures are prevalent in living systems and underpin numerous pivotal biological functions, yet their recapitulation in synthetic scenarios remains largely underexplored. Here, we report on compartmentalized supramolecular hydrogels that can dynamically evolve their structure and properties through chemically fueled self\u2010assembly in aqueous two\u2010phase systems (ATPSs) and uncover an unexpected dynamic interactive behavior between the hydrogel networks and ATPSs. By chemically fueling the self\u2010assembly of a simple peptide\u2010based gelator throughout aqueous emulsions of two immiscible polymer solutions, compartmentalized supramolecular hydrogel networks are generated. With the fuel dissipation, these hydrogels spontaneously disintegrate over time, with tunable lifetime and regeneration capacity. Interestingly, during the fueling process, the gelators are covalently decorated by one of the polymers in the ATPS, imparting the resultant hydrogel network with homotypic affinity for the corresponding polymer phase. This affinity drives an unexpected migration of the polymer phase, reminiscent of the migration of living cells assisted by the extracellular matrix. In turn, we leverage the polymer\u2010decorated gelator to control the compartmentalization regions of the hydrogel networks. This work would accelerate the exploitation of new supramolecular materials with lifelike features, including compartmentalized architectures, self\u2010evolving capacity, and interactive behaviors.<\/jats:p>","DOI":"10.1002\/smll.76277","type":"journal-article","created":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T13:13:59Z","timestamp":1791983639000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Compartmentalized Dynamic Supramolecular Hydrogels through Chemically Fueled Self\u2010Assembly in Aqueous Two\u2010Phase Systems"],"prefix":"10.1002","author":[{"given":"Guanyao","family":"Gu","sequence":"first","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuliang","family":"Gao","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingjing","family":"Chen","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qifeng","family":"Chang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kehong","family":"Lin","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8618-2594","authenticated-orcid":false,"given":"Zhongqi","family":"Li","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jan H.","family":"van Esch","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering Delft University of Technology  Delft The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1792-8564","authenticated-orcid":false,"given":"Xuhong","family":"Guo","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8269-8304","authenticated-orcid":false,"given":"Yiming","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering East China University of Science and Technology Shanghai China"},{"name":"Shanghai Key Laboratory for Intelligent Sensing and Detection Technology East China University of Science and Technology Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,14]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"crossref","first-page":"527","DOI":"10.1038\/nchembio.975","article-title":"Natural Strategies for the Spatial Optimization of Metabolism in Synthetic Biology","volume":"8","author":"Agapakis C. 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