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In this study, a regenerated cellulose nanofiber film (R\u2010CNF) is used as a substrate, and an aminosilane intermediate layer is introduced. By utilizing the silanol groups on the silane chains as compatible reactive sites for fluorination grafting, and simultaneously enhancing the bonding strength between modified layers through N\u2013H\u00b7\u00b7\u00b7F\u2013C hydrogen\u2010bond interactions between amino and fluorine groups, a fluorinated regenerated cellulose nanofiber film (F\u2010R\u2010CNF) is successfully prepared. The degradation rate of F\u2010R\u2010CNF within 13 days is approximately 0.96%. When assembled into a TENG with an ethyl cellulose nanofiber film(ECNF), the output voltage of the resulting TENG is ten times higher than that of the R\u2010CNF\u2010based TENGs, while maintaining 85% of its output performance at 80% relative humidity. Furthermore, a droplet energy harvesting TENG (DE\u2010TENG) is constructed to harvest energy from falling water droplets, demonstrating the potential of the DE\u2010TENG to power agricultural micro\u2010sensors. This study provides a feasible strategy for designing high\u2010performance all\u2010cellulose\u2010based triboelectric layer triboelectric nanogenerators and reveals the great potential of F\u2010R\u2010CNF for self\u2010powered devices and smart agriculture applications.<\/jats:p>","DOI":"10.1002\/smll.76354","type":"journal-article","created":{"date-parts":[[2026,10,19]],"date-time":"2026-10-19T11:57:22Z","timestamp":1792411042000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Triboelectric Nanogenerator Based on All\u2010Cellulose Triboelectric Layer for Droplet Energy Harvesting and Self\u2010Powered Agriculture Monitoring"],"prefix":"10.1002","author":[{"given":"Hengwei","family":"Xiong","sequence":"first","affiliation":[{"name":"College of Mechanical and Electrical Engineering Tarim University  Alar People's Republic of China"},{"name":"Modern Agricultural Engineering Key Laboratory at Universities of 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