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However, achieving stable and spatially uniform strain modulation remains challenging since conventional approaches are often constrained by compromised integrity, coherence\u2010strain trade\u2010offs, and defect\u2010induced charge recombination. Herein, we establish an adaptive amorphous\u2010crystalline interfacial coupling strategy that enables lattice strain engineering while concomitantly directing charge flow. By integrating hexagonal ZnIn\n                    <jats:sub>2<\/jats:sub>\n                    S\n                    <jats:sub>4<\/jats:sub>\n                    with amorphous CoO, spontaneous interfacial Co\u2500S bond formation and adaptive structural rearrangement of the amorphous phase cooperatively generate and stabilize uniform compressive strain within the crystalline lattice. The resulting compressive strain downshifts the\n                    <jats:italic>p<\/jats:italic>\n                    \u2010band center of surface sulfur atoms, optimizes the adsorption free energy of H\n                    <jats:sup>*<\/jats:sup>\n                    intermediates, and substantially lowers the kinetic barrier for the hydrogen evolution reaction. Meanwhile, interfacial Co\u2500S bonds, together with the built\u2010in electric field, establish an S\u2010scheme charge\u2010transfer pathway that directs photoexcited electrons toward catalytically active sulfur sites. Consequently, the amorphous\u2010crystalline heterostructure achieves a photocatalytic H\n                    <jats:sub>2<\/jats:sub>\n                    evolution rate of 24.9\u00a0mmol g\n                    <jats:sup>\u22121<\/jats:sup>\n                    h\n                    <jats:sup>\u22121<\/jats:sup>\n                    under simulated solar light and produces \u223c28\u00a0mL H\n                    <jats:sub>2<\/jats:sub>\n                    within 4\u00a0h under natural sunlight. These findings reveal amorphous\u2010crystalline interfaces as a versatile platform for coupling mechanical and electronic regulation in photocatalysis.\n                  <\/jats:p>","DOI":"10.1002\/smll.76400","type":"journal-article","created":{"date-parts":[[2026,10,21]],"date-time":"2026-10-21T11:13:08Z","timestamp":1792581188000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Adaptive Amorphous\u2010Crystalline Interfacial Coupling Enables Stable Lattice Strain Engineering for Enhanced Solar\u2010Driven H\n                    <sub>2<\/sub>\n                    Conversion"],"prefix":"10.1002","author":[{"given":"Shiting","family":"Wu","sequence":"first","affiliation":[{"name":"New Energy Materials Research Center College of Materials &amp; Environmental Engineering Hangzhou Dianzi University  Hangzhou Zhejiang People's Republic of 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