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Herein, this work presented a solvent\u2010free, transparent antifouling coating through room temperature vulcanization, based on a strategy of molecularly engineered nanocomposite networks. This strategy utilizes hydroxy\u2010terminated polydimethylsiloxane (HO\u2010PDMS\u2010OH) as functional segments to enable dynamic liquid repellency, isocyanatopropyltriethoxysilane (IPTS) and 3\u2010(2\u2010aminoethylamino) propylmethyldimethoxysilane (AEAPS) as dual cross\u2010linkers for rapid curing and robust network, and hydrophobic nano\u2010SiO2 as reinforcing fillers for anti\u2010fouling and mechanical robustness. The coating exhibited low VOC release through solvent\u2010free processing, high visible\u2010light transmittance (91% at 500\u00a0nm), and broad\u2010spectrum repellency with excellent durability against abrasion\/chemical exposure\/long\u2010term oil immersion. This unique coating strategy makes it possible for the ready application of antifouling technology onto heat\u2010sensitive, solvent\u2010sensitive, and flexible substrates such as flexible display devices. This work establishes an eco\u2010friendly paradigm for multifunctional protective coating through molecular nanocomposite engineering.<\/jats:p>","DOI":"10.1002\/smo2.70068","type":"journal-article","created":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T15:09:14Z","timestamp":1784646554000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Transparent, solvent\u2010free, and pressure\u2010tolerant antifouling coatings via molecular nanocomposite engineering"],"prefix":"10.1002","author":[{"given":"Jieran","family":"Li","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8571-4576","authenticated-orcid":false,"given":"Xiubin","family":"Xu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yueyan","family":"Liang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hongchun","family":"Mu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Xue","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianwei","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Daijiang","family":"Cai","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Lan","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiahui","family":"Tang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sizhe","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhenxuan","family":"Wei","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8907-6073","authenticated-orcid":false,"given":"Xu","family":"Wu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,7,21]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"crossref","first-page":"1134","DOI":"10.1038\/nbt.3020","volume":"32","author":"Leslie D. 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