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In this work, a metal\u2013organic framework\u2010based S\u2010scheme heterostructure (Ag<jats:sub>2<\/jats:sub>S@PB) is prepared to rapidly treat open wounds caused by bacterial infection, which effectively establishes and retains spatially isolated redox centers through an S\u2010scheme charge\u2010transfer pathway. Additionally, the formation of an interface electric field and covalent Fe\uf8ffS bridge bonding in the heterogeneous interface endows the heterojunction with a much stronger charge separation and transfer capability than bare Ag<jats:sub>2<\/jats:sub>S, which significantly enhances the photocatalytic performance and stability, consequently generating more radical oxygen species. Meanwhile, the introduction of Prussian blue greatly improves the photothermal effect of the Ag<jats:sub>2<\/jats:sub>S@PB under 808\u2009nm near\u2010infrared light. Therefore, under illumination for 20\u2009min, the Ag<jats:sub>2<\/jats:sub>S@PB shows a desirable antibacterial efficiency of 99.92% against <jats:italic>Staphylococcus aureus<\/jats:italic> and 99.86% against <jats:italic>Escherichia coli<\/jats:italic>. The in\u2009vivo wound repair experiment shows that the Ag<jats:sub>2<\/jats:sub>S@PB has good tissue repair effects and can expedite wound healing. This work will provide insights for designing highly efficient photoresponsive materials to treat bacterial wound infections.<\/jats:p>","DOI":"10.1002\/smsc.202300114","type":"journal-article","created":{"date-parts":[[2023,11,21]],"date-time":"2023-11-21T22:18:47Z","timestamp":1700605127000},"source":"Crossref","is-referenced-by-count":23,"title":["The Enhanced Photocatalytic Sterilization of a Metal\u2013Organic\u2010Framework\u2010Based S\u2010Scheme Heterostructure of Ag<sub>2<\/sub>S@PB for Rapid Healing of Bacteria\u2010Infected Open Wounds"],"prefix":"10.1002","volume":"3","author":[{"given":"Zhenxing","family":"Yang","sequence":"first","affiliation":[{"name":"Biomedical Materials Engineering Research Center Hubei Key Laboratory of Polymer Materials Ministry-of-Education Key Laboratory for the Green Preparation and Application of Functional Materials School of Materials Science &amp; Engineering Hubei University  Wuhan 430062 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