{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T03:08:55Z","timestamp":1791947335049,"version":"4.3.4"},"reference-count":44,"publisher":"Wiley","issue":"5","license":[{"start":{"date-parts":[[2024,2,9]],"date-time":"2024-02-09T00:00:00Z","timestamp":1707436800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100003052","name":"Ministry of Trade, Industry and Energy","doi-asserted-by":"publisher","id":[{"id":"10.13039\/501100003052","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Small Science"],"published-print":{"date-parts":[[2024,5]]},"abstract":"<jats:p>LiFePO<jats:sub>4<\/jats:sub>emerges as a viable alternative to cobalt\u2010containing cathodes, such as Li[Ni<jats:sub>1\u2013<jats:italic>x<\/jats:italic>\u2013<jats:italic>y<\/jats:italic><\/jats:sub>Mn<jats:sub><jats:italic>x<\/jats:italic><\/jats:sub>Co<jats:sub><jats:italic>y<\/jats:italic><\/jats:sub>]O<jats:sub>2<\/jats:sub>and Li[Ni<jats:sub>1\u2212<jats:italic>x<\/jats:italic>\u2212<jats:italic>y<\/jats:italic><\/jats:sub>Co<jats:sub><jats:italic>x<\/jats:italic><\/jats:sub>Al<jats:sub><jats:italic>y<\/jats:italic><\/jats:sub>]O<jats:sub>2<\/jats:sub>. As Fe is abundant in nature, LiFePO<jats:sub>4<\/jats:sub>is a low\u2010cost material. Moreover, stable structure of LiFePO<jats:sub>4<\/jats:sub>imparts long service life and thermal stability. However, the practical implementation of LiFePO<jats:sub>4<\/jats:sub>cathode in energy storage devices is impeded by its low energy density and high ionic\/electrical resistance. Herein, the LiFePO<jats:sub>4<\/jats:sub>electrode with high active material loading and low ionic\/electrical resistance through the dry process is reported for the first time. The dry process not only enables the uniform distribution of the polymeric binders and conductive additives within the thick electrode but also inhibits the formation of cracks. Furthermore, the bridge\u2010like connection of polytetrafluoroethylene facilitates the insertion and extraction of Li ions to the LiFePO<jats:sub>4<\/jats:sub>crystal. Hence, the dry\u2010processed LiFePO<jats:sub>4<\/jats:sub>electrode with high areal capacity (7.8\u2009mAh\u2009cm<jats:sup>\u22122<\/jats:sup>) exhibits excellent cycle stability over 300 cycles in full\u2010cell operation. In addition, it is demonstrated that the estimated energy density of prismatic cell with the dry\u2010processed LiFePO<jats:sub>4<\/jats:sub>electrode is competitive with state\u2010of\u2010the\u2010art Li[Ni<jats:sub>1\u2013<jats:italic>x<\/jats:italic>\u2013<jats:italic>y<\/jats:italic><\/jats:sub>Mn<jats:sub><jats:italic>x<\/jats:italic><\/jats:sub>Co<jats:sub><jats:italic>y<\/jats:italic><\/jats:sub>]O<jats:sub>2<\/jats:sub>\u2010based battery.<\/jats:p>","DOI":"10.1002\/smsc.202300302","type":"journal-article","created":{"date-parts":[[2024,2,9]],"date-time":"2024-02-09T19:54:19Z","timestamp":1707508459000},"source":"Crossref","is-referenced-by-count":99,"title":["Low\u2010Resistance LiFePO<sub>4<\/sub>Thick Film Electrode Processed with Dry Electrode Technology for High\u2010Energy\u2010Density Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"4","author":[{"given":"Kihwan","family":"Kwon","sequence":"first","affiliation":[{"name":"Energy Storage Materials Center Korea Institute of Ceramic Engineering and Technology Jinju 52851 Republic of Korea"},{"name":"Department of Applied Chemistry Kyungpook National University Daegu 41566 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiwoon","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Energy Engineering Hanyang University 222 Wangsimni\u2010ro Seoul 04763 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Seungmin","family":"Han","sequence":"additional","affiliation":[{"name":"Energy Storage Materials Center Korea Institute of Ceramic Engineering and Technology Jinju 52851 Republic of Korea"},{"name":"Department of Energy Engineering Hanyang University 222 Wangsimni\u2010ro Seoul 04763 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Joohyun","family":"Lee","sequence":"additional","affiliation":[{"name":"Energy Storage Materials Center Korea Institute of Ceramic Engineering and Technology Jinju 52851 Republic of Korea"},{"name":"Department of Materials Science and Engineering Pusan National University Pusan 46241 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hyungjun","family":"Lee","sequence":"additional","affiliation":[{"name":"Department of Energy Engineering Hanyang University 222 Wangsimni\u2010ro Seoul 04763 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiseok","family":"Kwon","sequence":"additional","affiliation":[{"name":"Department of Energy Engineering Hanyang University 222 Wangsimni\u2010ro Seoul 04763 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jungwoo","family":"Lee","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering Pusan National University Pusan 46241 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jihoon","family":"Seo","sequence":"additional","affiliation":[{"name":"Department of Chemical &amp; Biomolecular Engineering Clarkson University Potsdam NY 13699 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Patrick Joohyun","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Applied Chemistry Kyungpook National University Daegu 41566 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Taeseup","family":"Song","sequence":"additional","affiliation":[{"name":"Department of Energy Engineering Hanyang University 222 Wangsimni\u2010ro Seoul 04763 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4577-7967","authenticated-orcid":false,"given":"Junghyun","family":"Choi","sequence":"additional","affiliation":[{"name":"Energy Storage Materials Center Korea Institute of Ceramic Engineering and Technology Jinju 52851 Republic of Korea"},{"name":"Department of Battery Engineering Gachon University 1342, Seongnam\u2010daero, Sujeong\u2010gu Seongnam\u2010si Gyeonggi\u2010do Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,2,9]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0EE03581E"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ensm.2023.102899"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.energyfuels.1c03757"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.elecom.2023.107558"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.3390\/nano13010090"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.3390\/batteries8100133"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.isci.2021.102787"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1109\/ACCESS.2022.3182726"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2019.02.114"},{"key":"e_1_2_8_11_1","doi-asserted-by":"crossref","unstructured":"A.Barai W. D.Widanage A.McGordon P.Jennings in2016 IEEE Transportation Electrification Conf. and Expo (ITEC) IEEE Dearborn MI2016 pp.1\u20134.","DOI":"10.1109\/ITEC.2016.7520299"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.3390\/batteries7030051"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2022.140464"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1021\/accountsmr.1c00281"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201901457"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1039\/D2EE03840D"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-023-37009-7"},{"key":"e_1_2_8_18_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsenergylett.3c00936"},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1002\/er.8266"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.matt.2022.01.011"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2022.04.008"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.3390\/nano13111771"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1021\/am404580f"},{"key":"e_1_2_8_24_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41598-019-51474-5"},{"key":"e_1_2_8_25_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsaem.1c02334"},{"key":"e_1_2_8_26_1","doi-asserted-by":"publisher","DOI":"10.1149\/1945-7111\/ab9404"},{"key":"e_1_2_8_27_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-017-02291-9"},{"key":"e_1_2_8_28_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.elecom.2023.107598"},{"key":"e_1_2_8_29_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2021.230219"},{"key":"e_1_2_8_30_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.jpclett.8b02229"},{"key":"e_1_2_8_31_1","doi-asserted-by":"publisher","DOI":"10.1002\/batt.202300170"},{"key":"e_1_2_8_32_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2023.233238"},{"key":"e_1_2_8_33_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.jpcc.9b11929"},{"key":"e_1_2_8_34_1","doi-asserted-by":"publisher","DOI":"10.3390\/batteries7040070"},{"key":"e_1_2_8_35_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2016.04.018"},{"key":"e_1_2_8_36_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.matdes.2022.111208"},{"key":"e_1_2_8_37_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsaem.9b01695"},{"key":"e_1_2_8_38_1","doi-asserted-by":"publisher","DOI":"10.3390\/batteries9030151"},{"key":"e_1_2_8_39_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.2c15685"},{"key":"e_1_2_8_40_1","doi-asserted-by":"publisher","DOI":"10.1038\/srep23150"},{"key":"e_1_2_8_41_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9TA08299A"},{"key":"e_1_2_8_42_1","doi-asserted-by":"publisher","DOI":"10.3390\/en14071902"},{"key":"e_1_2_8_43_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2004.06.059"},{"key":"e_1_2_8_44_1","doi-asserted-by":"publisher","DOI":"10.1149\/2.1021814jes"},{"key":"e_1_2_8_45_1","doi-asserted-by":"publisher","DOI":"10.1002\/batt.202100224"}],"container-title":["Small Science"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/smsc.202300302","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2024,11,10]],"date-time":"2024-11-10T23:50:38Z","timestamp":1731282638000},"score":1,"resource":{"primary":{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/smsc.202300302"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2024,2,9]]},"references-count":44,"journal-issue":{"issue":"5","published-print":{"date-parts":[[2024,5]]}},"alternative-id":["10.1002\/smsc.202300302"],"URL":"https:\/\/doi.org\/10.1002\/smsc.202300302","archive":["Portico"],"relation":{},"ISSN":["2688-4046","2688-4046"],"issn-type":[{"value":"2688-4046","type":"print"},{"value":"2688-4046","type":"electronic"}],"subject":[],"published":{"date-parts":[[2024,2,9]]},"article-number":"2300302"}}