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Metal organic frameworks (MOFs)\u2010based membrane separation technology has demonstrated to be an efficient and sustainable approach for CO\n                    <jats:sub>2<\/jats:sub>\n                    separation and capture compared to the conventional methods. The development of high\u2010performance materials and fabrication techniques, assisted with modern computational methods, has become an active research area. In this review, the state of the art and applications of MOFs\u2010based membrane for CO\n                    <jats:sub>2<\/jats:sub>\n                    separation technology were summarized, and the materials synthesis and modification methods reported in the last five years were comprehensively compared to evaluate the advantages and limitations in improving the permeability and selectivity of the membranes. The most recent progress of computational methods involving molecular simulations and machine learning was outlined to understand the underlying molecular mechanisms of the separation performance and high\u2010throughput screening of materials. Finally, the challenges and prospects of the current development status of MOFs\u2010based membranes in both experiments and data\u2010driven methods for CO\n                    <jats:sub>2<\/jats:sub>\n                    separation were addressed.\n                  <\/jats:p>","DOI":"10.1002\/smtd.202502117","type":"journal-article","created":{"date-parts":[[2026,1,30]],"date-time":"2026-01-30T06:32:37Z","timestamp":1769754757000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Enhancing the CO\n                    <sub>2<\/sub>\n                    Separation Performance of MOFs\u2010Based Membranes: From Strategic Modifications to Computational Insights"],"prefix":"10.1002","volume":"10","author":[{"given":"Xiaohui","family":"Liu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Shanghai Institute of Pollution Control and Ecological Security Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zixuan","family":"Yu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Shanghai Institute of Pollution Control and Ecological Security Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haochen","family":"Zhu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Shanghai Institute of Pollution Control and Ecological Security Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenquan","family":"Tao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Shanghai Institute of Pollution Control and Ecological Security Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7452-7030","authenticated-orcid":false,"given":"Zhuo","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Shanghai Institute of Pollution Control and Ecological Security Tongji University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Boyu","family":"Li","sequence":"additional","affiliation":[{"name":"Department of Environmental and Sustainable Engineering University at Albany State University of New York  Albany New York United States"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Aziz","family":"Ghoufi","sequence":"additional","affiliation":[{"name":"Univ Paris\u2010East Creteil CNRS ICMPE (UMR7182)  Thiais 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