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However, the slow iodine conversion, polyiodide shuttle effect, and uncontrollable Zn dendrites impede the improvement of their performance. Herein, we successfully designed a bifunctional core\u2013shell host derived from BiHCF@ZIF\u20108, which consists of a porous carbon matrix encapsulating abundant metal catalytic sites and trace N\u2010doping (BZPC). This superior multi\u2010site co\u2010doped hierarchical porous structure can serve as a high\u2010efficiency iodine carrier to effectively confine iodine species and enhance their conversion kinetics. Simultaneously, the BZPC can also be applied as a functional modification layer to induce uniform Zn deposition, thereby achieving a dendrite\u2010free Zn anode. The assembled Zn\/\/BZPC@I\n                    <jats:sub>2<\/jats:sub>\n                    batteries and BZPC@Zn symmetric cells can operate stably at ultrahigh current densities of 50\u00a0C and 100\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , respectively. Through a synergistic optimization strategy of \u201cone host for dual purposes\u201d, the BZPC@Zn\/\/BZPC@I\n                    <jats:sub>2<\/jats:sub>\n                    batteries achieve an ultralong lifespan of 28\u00a0000 stable cycles even at an ultrahigh current density of 50\u00a0C. This study not only pioneers the difunctional BZPC for both iodine host design and zinc interface engineering but also establishes an innovative and scalable strategy for developing long\u2010life and high\u2010rate Zn\u2500I\n                    <jats:sub>2<\/jats:sub>\n                    batteries.\n                  <\/jats:p>","DOI":"10.1002\/smtd.202502240","type":"journal-article","created":{"date-parts":[[2026,1,10]],"date-time":"2026-01-10T14:06:18Z","timestamp":1768053978000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Multi\u2010Site Co\u2010Doped Hierarchical Porous Carbon for Efficient Iodine Conversion and Uniform Zinc Deposition in Zinc\u2013Iodine Batteries"],"prefix":"10.1002","volume":"10","author":[{"given":"Qiushao","family":"Yang","sequence":"first","affiliation":[{"name":"College of Materials Science and Engineering Nanjing Tech University  Nanjing 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