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Metal\u2013organic frameworks (MOFs) have emerged as highly promising materials for sensing applications owing to their high porosity, structural diversity, tunable pore architectures, and tailorable host\u2013guest interactions. However, the practical deployment of MOF powders in sensing devices is often limited by poor processability, random particle packing, and insufficient compatibility with device fabrication. In contrast, surface\u2010mounted metal\u2013organic frameworks (SURMOFs), as highly ordered MOF thin films grown directly on substrates, offer unique advantages for constructing advanced sensing platforms, including controlled orientation, tunable thickness, patterned growth, and excellent compatibility with device integration. In this review, we summarize recent progress in SURMOF\u2010based advanced sensing applications, with emphasis on their fabrication strategies and representative applications in various types of sensors. 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