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These conditions intensify the coupling among ion transport, interfacial reactions, and the limited inventories of electrolyte and active lithium, leading to transport polarization, unstable electrode\u2010electrolyte interphases, and irreversible material loss. Although electrolyte design has evolved from empirical formulation optimization to coordinated regulation across solvation, molecular, interfacial, and system levels, systematic links between condition\u2010specific failure mechanisms and corresponding design strategies remain incomplete. This review elucidates dynamic Li\n                    <jats:sup>+<\/jats:sup>\n                    solvation dynamics, multiscale transport, interphase evolution, and electrolyte and active\u2010lithium consumption govern cycling stability under extreme conditions. Representative strategies, including solvation and transport regulation, molecular and interfacial reaction engineering, polymer\/gel electrolytes, and spatially differentiated electrolytes, are summarized with emphasis on their operating windows and trade\u2010offs. Finally, we propose that electrolyte design under extreme conditions should identify the dominant condition\u2010specific limitation and coordinate solvation, transport, interfacial reactions, and the consumption of electrolyte and active lithium accordingly, thereby establishing an integrated \u201capplication conditions\u2013failure mechanisms\u2013key descriptors\u2013electrolyte engineering\u2013practical validation\u201d framework for practical high\u2010specific\u2010energy LMBs.\n                  <\/jats:p>","DOI":"10.1002\/adfm.78881","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T11:58:30Z","timestamp":1791374310000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Electrolyte Engineering for Lithium Metal Batteries Under Extreme Operating Conditions"],"prefix":"10.1002","author":[{"given":"Zhen","family":"Wang","sequence":"first","affiliation":[{"name":"School of Materials and Energy University of Electronic Science and Technology of China  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kewen","family":"Chen","sequence":"additional","affiliation":[{"name":"College of Materials and Chemistry &amp; Chemical Engineering (College of Lithium Resources and Lithium Battery Industry) Chengdu University of Technology  Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-9543-1861","authenticated-orcid":false,"given":"Fei","family":"Li","sequence":"additional","affiliation":[{"name":"School of Materials and Energy University of Electronic Science and Technology of China  Chengdu China"},{"name":"Energy and Information Materials Key Laboratory of Sichuan Province University of Electronic Science and Technology of China  Chengdu 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