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Here, maintaining structural\/electrode stability against large volume change by means of an all\u2010integrated design is realized for silicon anodes. An all\u2010integrated silicon anode is achieved via multicomponent interlinking among carbon@void@silica@silicon (CVSS) nanospheres and cross\u2010linked carboxymethyl cellulose and citric acid polymer binder (c\u2010CMC\u2010CA). Due to the additional protection from the silica layer, CVSS is superior to the carbon@void@silicon (CVS) electrode in terms of long\u2010term cyclability. The as\u2010prepared all\u2010integrated CVSS electrode exhibits high mechanical strength, which can be ascribed to the high adhesivity and ductility of c\u2010CMC\u2010CA binder and the strong binding energy between CVSS and c\u2010CMC\u2010CA, as calculated based on density functional theory (DFT). This electrode exhibits a high reversible capacity of 1640 mA h g<jats:sup>\u22121<\/jats:sup> after 100 cycles at a current density of 1 A g<jats:sup>\u22121<\/jats:sup>, high rate performance, and long\u2010term cycling stability with 84.6% capacity retention after 1000 cycles at 5 A g<jats:sup>\u22121<\/jats:sup>.<\/jats:p>","DOI":"10.1002\/adma.201703028","type":"journal-article","created":{"date-parts":[[2017,10,12]],"date-time":"2017-10-12T15:24:43Z","timestamp":1507821883000},"source":"Crossref","is-referenced-by-count":296,"title":["An All\u2010Integrated Anode via Interlinked Chemical Bonding between Double\u2010Shelled\u2013Yolk\u2010Structured Silicon and Binder for Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"29","author":[{"given":"Yajie","family":"Liu","sequence":"first","affiliation":[{"name":"Institute for Superconducting and Electronic Materials Australian Institute for Innovative Materials University of Wollongong  Innovation Campus North Wollongong NSW 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