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The focus is on synergies that prioritize sustainability and environmental benefits. This study explores the potential of abundant, non\u2010toxic, and sustainable resources such as paper, lignin\u2010enriched paper, and cork for producing laser\u2010induced graphene (LIG) supercapacitor electrodes with improved capacitance. A single\u2010step methodology using a CO<jats:sub>2<\/jats:sub> laser system is developed for fabricating these electrodes under ambient conditions, providing an environmentally friendly alternative to conventional carbon sources. The resulting green micro\u2010supercapacitors (MSCs) achieve impressive areal capacitance (\u22487\u201310 mF cm<jats:sup>\u22122<\/jats:sup>) and power and energy densities (\u22484 \u03bcW cm<jats:sup>\u20102<\/jats:sup> and \u22480.77 \u00b5Wh cm<jats:sup>\u22122<\/jats:sup> at 0.01\u00a0mA cm<jats:sup>\u22122<\/jats:sup>). Stability tests conducted over 5000 charge\u2013discharge cycles demonstrate a capacitance retention of \u224880\u201385%, highlighting the device durability. These LIG\u2010based devices offer versatility, allowing voltage output adjustment through stacked and sandwich MSCs configurations (parallel or series), suitable for various large\u2010scale applications. This study demonstrates that it is possible to create high\u2010quality energy storage devices based on biodegradable materials. This development can lead to progress in renewable energy and off\u2010grid technology, as well as a reduction in electronic waste.<\/jats:p>","DOI":"10.1002\/admt.202400261","type":"journal-article","created":{"date-parts":[[2024,5,17]],"date-time":"2024-05-17T02:39:30Z","timestamp":1715913570000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":24,"title":["Green Fabrication of Stackable Laser\u2010Induced Graphene Micro\u2010Supercapacitors under Ambient Conditions: Toward the Design of Truly Sustainable Technological Platforms"],"prefix":"10.1002","volume":"9","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3560-4317","authenticated-orcid":false,"given":"Sara L.","family":"Silvestre","sequence":"first","affiliation":[{"name":"CENIMAT i3N Department of Materials Science School of Science and Technology NOVA University Lisbon and CEMOP\/UNINOVA  Caparica Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3527-7857","authenticated-orcid":false,"given":"Maria","family":"Morais","sequence":"additional","affiliation":[{"name":"CENIMAT i3N Department of Materials Science School of Science and Technology NOVA University Lisbon and CEMOP\/UNINOVA  Caparica Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4867-7390","authenticated-orcid":false,"given":"Raquel R. 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