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In this work, the valorization of <jats:italic>Eucalyptus globulus<\/jats:italic> wood, a forest invasive species present in European forests, is performed through its transformation in biochar. The deposition of nitrogen and different metals (aluminum, copper and chromium) onto biochar is performed, using the magnetron sputtering as a pioneering technique, to produce coated biochar nanoparticles with improved properties. The resultant modified biochar particles maintain a highly porous structure and present a remarkable CO<jats:sub>2<\/jats:sub> adsorption capacity (up to 4.80\u00a0mmol\u00a0g<jats:sup>\u22121<\/jats:sup> for <jats:bold>N@BC<\/jats:bold>), which is attributed to the synergy of their large total surface area (527\u00a0m<jats:sup>2<\/jats:sup>\u00a0g<jats:sup>\u22121<\/jats:sup>) and microporosity (pore diameter = 21\u00a0\u00c5), with a high content of nitrogen and oxygen heteroatom moieties (40.4% N, 11.4% O). Their application as heterogeneous bifunctional catalysts in CO<jats:sub>2<\/jats:sub> cycloaddition to epichlorohydrin is performed, in the absence of any solvent or co\u2010catalyst, under moderate conditions (20\u00a0bar CO<jats:sub>2<\/jats:sub>, 120\u00a0\u00b0C), leading to good conversions (up to 58% conversion) and excellent selectivity for cyclic carbonates. Cu\u2010coated biochar is shown to be more stable than non\u2010modified material, being recycled and reused along 4 consecutive runs without loss of catalytic activity or selectivity.<\/jats:p>","DOI":"10.1002\/adsu.202400431","type":"journal-article","created":{"date-parts":[[2024,10,9]],"date-time":"2024-10-09T03:00:56Z","timestamp":1728442856000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Modified Biochar Materials From <i>Eucalyptus globulus<\/i> Wood as Efficient CO<sub>2<\/sub> Adsorbents and Recyclable Catalysts"],"prefix":"10.1002","volume":"9","author":[{"given":"Shahab","family":"Zomorodbakhsh","sequence":"first","affiliation":[{"name":"Department of Chemistry CQC \u2013 Coimbra Chemistry Centre University of Coimbra  Rua Larga 2 Coimbra 3004\u2013535 Portugal"}]},{"given":"Andreia C. 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