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The obtained materials were tested for the oxidation of cyclohexane under mild conditions (room temperature and atmospheric pressure), using an environmentally friendly oxidant (<jats:italic>tert<\/jats:italic>\u2010butyl hydroperoxide, TBHP, 70\u2009% aqueous solution). All materials were very selective to the production of cyclohexanol and cyclohexanone with no trace of by\u2010products detected. The catalysts were also tested in the selective oxidation of methyl benzyl alcohol, cyclohexanol, and 2\u2010octanol with TBHP, under microwave irradiation, to the corresponding aldehydes or ketones. In general, better results are obtained for the heterogenised complexes and that the most efficient support is CNT\u2010ox\u2010Na. This is the first report on the oxidation of C\u2212H bonds using the mononuclear gold complexes used; only the oxidation of unsaturated units had been reported previously. The sp<jats:sup>3<\/jats:sup>\u2010C\u2212H activation is much more difficult than the oxidation of unsaturated molecules with molecular oxidants.<\/jats:p>","DOI":"10.1002\/cctc.201701886","type":"journal-article","created":{"date-parts":[[2018,1,3]],"date-time":"2018-01-03T11:52:26Z","timestamp":1514980346000},"page":"1804-1813","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":26,"title":["Commercial Gold(I) and Gold(III) Compounds Supported on Carbon Materials as Greener Catalysts for the Oxidation of Alkanes and Alcohols"],"prefix":"10.1002","volume":"10","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9913-4671","authenticated-orcid":false,"given":"S\u00f3nia A. 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