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Complexes <jats:bold>1<\/jats:bold>\u2013<jats:bold>3<\/jats:bold> were characterized by elemental analysis, IR spectroscopy, single\u2010crystal X\u2010ray crystallography, electrochemical methods and variable\u2010temperature magnetic susceptibility measurements, which indicated that the intratrimer antiferromagnetic coupling is strong in the three complexes and that there exists very weak ferromagnetic intermolecular interactions in <jats:bold>1<\/jats:bold> but weak antiferromagnetic intermolecular interactions in both <jats:bold>2<\/jats:bold> and <jats:bold>3<\/jats:bold>. Electrochemical experiments showed that in complexes <jats:bold>1<\/jats:bold>\u2013<jats:bold>3<\/jats:bold> the Cu<jats:sup>II<\/jats:sup> ions can be reduced, in distinct steps, to Cu<jats:sup>I<\/jats:sup> and Cu<jats:sup>0<\/jats:sup>. All the complexes act as efficient catalyst precursors under mild conditions for the peroxidative oxidation of cyclohexane to cyclohexyl hydroperoxide, cyclohexanol and cyclohexanone, leading to overall yields (based on the alkane) of up to 31\u2009% (TON = 1.55\u2009\u00d7\u200910<jats:sup>3<\/jats:sup>) after 6 h in the presence of pyrazinecarboxylic acid.<\/jats:p>","DOI":"10.1002\/ejic.201500440","type":"journal-article","created":{"date-parts":[[2015,7,19]],"date-time":"2015-07-19T11:33:19Z","timestamp":1437305599000},"page":"3959-3969","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":53,"title":["Trinuclear Cu<sup>II<\/sup> Structural Isomers: Coordination, Magnetism, Electrochemistry and Catalytic Activity towards the Oxidation of Alkanes"],"prefix":"10.1002","volume":"2015","author":[{"given":"Manas","family":"Sutradhar","sequence":"first","affiliation":[]},{"given":"Lu\u00edsa M. D. R. 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