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Most of the works exploit the hyperfine properties, Electric Field Gradient (EFG) and Hyperfine Magnetic Field (HMF), of these probes through Perturbed Angular Correlation (PAC) spectroscopy. The measurements were complemented with density functional theory calculations to model the relevant properties and correlate the EFG with the electric polarization. We also present a methodological and nuclear physics related contribution consisting on the characterization of a new short\u2010lived isotope adequate for PAC studies. Finally, an ultra\u2010sensitive method to quantify the uptake of Hg by nano sorbents based on the tracking the radioactive isotopes of mercury is also reviewed. These works showcase the diversity of our research with radioisotopes, at the interface of different science fields, with combination of different methodologies and different motivations such as fundamental materials physics and chemistry or environmental concerns.<\/jats:p>","DOI":"10.1002\/ejic.202000047","type":"journal-article","created":{"date-parts":[[2020,3,27]],"date-time":"2020-03-27T16:49:48Z","timestamp":1585327788000},"page":"1822-1833","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Exploiting Radioactive Isotopes: from Pollutant Tracking to Solid State Studies Using a Combined <i>Ab Initio<\/i> and PAC Approach"],"prefix":"10.1002","volume":"2020","author":[{"given":"Carlos O.","family":"Amorim","sequence":"first","affiliation":[{"name":"CICECO Aveiro Institute of Materials and Physics Department University of Aveiro Physics Department  3810\u2010193 Aveiro Portugal"}]},{"given":"Jo\u00e3o N.","family":"Gon\u00e7alves","sequence":"additional","affiliation":[{"name":"CICECO Aveiro Institute of Materials and Physics Department University of Aveiro Physics Department  3810\u2010193 Aveiro Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3359-7133","authenticated-orcid":false,"given":"V\u00edtor S.","family":"Amaral","sequence":"additional","affiliation":[{"name":"CICECO Aveiro Institute of Materials and Physics Department University of Aveiro Physics Department  3810\u2010193 Aveiro Portugal"}]}],"member":"311","published-online":{"date-parts":[[2020,4,24]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmmm.2003.12.1134"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.73.100408"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/25\/38\/385602"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/pssb.201350075"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmmm.2003.12.957"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.100.155702"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jnoncrysol.2008.06.124"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.72.144523"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.84.094524"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmmm.2009.06.079"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/26\/21\/215401"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1051\/epjconf\/20147509002"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.83.104421"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.86.035145"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1007\/s10751-010-0233-0"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.microc.2018.01.039"},{"key":"e_1_2_8_18_1","unstructured":"ISOLDE radioactive ion beam facility http:\/\/isolde.web.cern.ch."},{"volume-title":"Nuclear condensed matter physics. 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