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Current research in this field remains exploratory because there is a lack of standards, methods, and policies for the detection, removal, and regulation of MPs discharge. In this study, a series of metal\u2013organic framework (MOFs)-incorporated hydrogels was successfully fabricated via a photo-initiated cross-linking strategy, offering a facile and efficient preparation approach applicable to the removal of diverse MPs types. Among them, ZIF\u20138.1@H6mg exhibited the highest MPs removal efficiencies, achieving up to 97% for polyethylene terephthalate (PET) and 98% for polyethylene (PE) in laundry wastewater, one of the main sources of MPs pollution. The material demonstrated excellent recyclability, with MPs removal efficiency only slightly decreasing to 96% after six reuse cycles. It maintained stable operation for approximately 4\u00a0h, and pre-treatment with backwashing further enhanced long-term filtration performance. Comprehensive characterization of the ZIF-8 hydrogel composites suggests that their interpenetrating network structures, zeta potential, and surface functional groups contributed to their superior performance. These findings highlight the potential of ZIF-based hydrogels as sustainable and effective materials for mitigating the growing threat of MPs pollution.<\/jats:p>","DOI":"10.1007\/s11356-026-38156-2","type":"journal-article","created":{"date-parts":[[2026,9,1]],"date-time":"2026-09-01T06:52:32Z","timestamp":1788245552000},"page":"14165-14177","update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Synthesis of metal organic framework-based hydrogel for microplastics removal from aquatic environments"],"prefix":"10.1007","volume":"33","author":[{"given":"Thi Trang","family":"Luu","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shudi","family":"Mao","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dai Quyet","family":"Truong","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yihan","family":"Shi","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Thi Ngoc Oanh","family":"Duong","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qiang","family":"Fu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Van Manh","family":"Do","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Saravanamuthu","family":"Vigneswaran","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3893-1217","authenticated-orcid":false,"given":"Tien Vinh","family":"Nguyen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,9,1]]},"reference":[{"key":"38156_CR1","doi-asserted-by":"crossref","unstructured":"Ahmad, M., Patel, R., Lee, D. 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