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However, its rate performance and cycling stability are poor due to the severe particle pulverization during the lithiation\/delithiation process. The high stress induced by the Li concentration gradient and anisotropic deformation is the main reason for the fracture of Si particles. Here we present a new stress mitigation strategy by uniformly distributing small amounts of Sn and Sb in Si micron-sized particles, which reduces the Li concentration gradient and realizes an isotropic lithiation\/delithiation process. The Si<jats:sub>8.5<\/jats:sub>Sn<jats:sub>0.5<\/jats:sub>Sb microparticles (mean particle size: 8.22\u00a0\u03bcm) show over 6000-fold and tenfold improvements in electronic conductivity and Li diffusivity than Si particles, respectively. The discharge capacities of the Si<jats:sub>8.5<\/jats:sub>Sn<jats:sub>0.5<\/jats:sub>Sb microparticle anode after 100 cycles at 1.0 and 3.0\u00a0A\u00a0g<jats:sup>\u22121<\/jats:sup> are 1.62 and 1.19\u00a0Ah\u00a0g<jats:sup>\u22121<\/jats:sup>, respectively, corresponding to a retention rate of 94.2% and 99.6%, respectively, relative to the capacity of the first cycle after activation. Multicomponent microparticle anodes containing Si, Sn, Sb, Ge and Ag prepared using the same method yields an ultra-low capacity decay rate of 0.02% per cycle for 1000 cycles at 1\u00a0A\u00a0g<jats:sup>\u22121<\/jats:sup>, corroborating the proposed mechanism. The stress regulation mechanism enabled by the industry-compatible fabrication methods opens up enormous opportunities for low-cost and high-energy\u2013density Li-ion batteries.<\/jats:p>","DOI":"10.1007\/s40820-023-01190-7","type":"journal-article","created":{"date-parts":[[2023,10,9]],"date-time":"2023-10-09T08:42:48Z","timestamp":1696840968000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":68,"title":["High-Performance Silicon-Rich Microparticle Anodes for Lithium-Ion Batteries Enabled by Internal Stress Mitigation"],"prefix":"10.1007","volume":"15","author":[{"given":"Yao","family":"Gao","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lei","family":"Fan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rui","family":"Zhou","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoqiong","family":"Du","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zengbao","family":"Jiao","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Biao","family":"Zhang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2023,10,9]]},"reference":[{"issue":"7411","key":"1190_CR1","doi-asserted-by":"publisher","first-page":"294","DOI":"10.1038\/nature11475","volume":"488","author":"S Chu","year":"2012","unstructured":"S. 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