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Moreover, rechargeable nonaqueous metal\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    batteries have attracted much attention due to their high theoretical energy density. However, the stability issues of the electrode\u2013electrolyte interfaces of nonaqueous metal\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    (lithium (Li)\/sodium (Na)\/potassium (K)\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    ) batteries have been troubling its development, and a large number of related research in the field of electrolytes have conducted in recent years. This review retraces the short but rapid research history of nonaqueous metal\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    batteries with a detailed electrochemical mechanism analysis. Then it focuses on the basic characteristics and design principles of electrolytes, summarizes the latest achievements of various types of electrolytes in a timely manner and deeply analyzes the construction strategies of stable electrode\u2013electrolyte interfaces for metal\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    batteries. Finally, the key issues related to electrolytes and interface engineering are fully discussed and several potential directions for future research are proposed. This review enriches a comprehensive understanding of electrolytes and interface engineering toward the practical applications of next-generation metal\u2013CO\n                    <jats:sub>2<\/jats:sub>\n                    batteries.\n                  <\/jats:p>","DOI":"10.1007\/s40820-025-01801-5","type":"journal-article","created":{"date-parts":[[2025,6,15]],"date-time":"2025-06-15T23:52:56Z","timestamp":1750031576000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":19,"title":["Understanding Electrolytes and Interface Chemistry for Sustainable Nonaqueous Metal\u2013CO2 Batteries"],"prefix":"10.1007","volume":"17","author":[{"given":"Bijiao","family":"He","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yunnian","family":"Ge","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fang","family":"Zhang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huajun","family":"Tian","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yan","family":"Xin","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yong","family":"Lei","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Yang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2025,6,16]]},"reference":[{"issue":"21","key":"1801_CR1","doi-asserted-by":"publisher","first-page":"5785","DOI":"10.1002\/anie.201701928","volume":"56","author":"X Hu","year":"2017","unstructured":"X. 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