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Here, we report noble metal-doped NiV layered double hydroxides (LDHs) that integrate electronic modulation with a dual chloride confinement mechanism. Ir incorporation simultaneously establishes strong Ir-Cl coordination and dynamically regenerated VO\n                    <jats:sub>4<\/jats:sub>\n                    <jats:sup>3\u2212<\/jats:sup>\n                    layers, producing an adaptive electrostatic shield that effectively suppresses chloride penetration. As a result, Ir-NiV LDH delivers nearly 100% oxygen evolution reaction selectivity and outstanding stability over 2750 h at 500 mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . Meanwhile, Ru doping optimizes the hydrogen evolution pathway, enabling a low overpotential of 195 mV and &gt;2350 h durability. When paired in a twso-electrode electrolyzer, the Ru-NiVLDH||Ir-NiVLDH system exhibits industrial-level performance and unprecedented robustness in alkaline seawater. This dual chloride confinement concept provides a general framework for catalyst design in corrosive ionic environments, extending beyond seawater splitting toward other electrochemical energy conversion processes.\n                  <\/jats:p>","DOI":"10.1007\/s40820-026-02067-1","type":"journal-article","created":{"date-parts":[[2026,1,16]],"date-time":"2026-01-16T09:28:03Z","timestamp":1768555683000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":27,"title":["Dual Chloride Confinement in Noble Metal\u2010Doped NiV LDH Catalysts Enables Stable Industrial-Level Seawater Electrolysis"],"prefix":"10.1007","volume":"18","author":[{"given":"Kai","family":"Liu","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yaohai","family":"Cai","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaotian","family":"Wei","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lihang","family":"Qu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianxi","family":"Lu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yingwei","family":"Qi","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhenbo","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dong","family":"Liu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,1,16]]},"reference":[{"issue":"7941","key":"2067_CR1","doi-asserted-by":"publisher","first-page":"673","DOI":"10.1038\/s41586-022-05379-5","volume":"612","author":"H Xie","year":"2022","unstructured":"H. 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