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This study develops a gradient-laminated ceramifiable silicone foam composite to resolve the inherent trade-off between thermal insulation and dynamic impact toughness. By integrating a polydimethylsiloxane foam matrix with a load-bearing glass fiber fabric skeleton, the material utilizes silane coupling agents for robust interfacial adhesion, while multiscale fillers promote synergistic ceramicization. Characterization reveals robust mechanical durability, maintaining stable elasticity across a wide temperature range (\u2212\u200940 to 300\u00a0\u00b0C) and retaining 93% residual stress after 1,000 compression cycles. Under extreme thermal exposure, the foam transforms into a dense ceramic barrier, reducing total heat release by 54.4% and sustaining thermal protection for over 30\u00a0min. Crucially, during battery module testing, this architecture efficiently intercepts high-velocity gas jets and confines thermal runaway to a single cell. Fabricated via a scalable process, this composite paves a viable way for constructing intrinsically safe energy storage systems.<\/jats:p>","DOI":"10.1007\/s40820-026-02228-2","type":"journal-article","created":{"date-parts":[[2026,5,24]],"date-time":"2026-05-24T10:10:26Z","timestamp":1779617426000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Constructing Intrinsically Safe Lithium-Ion Battery Energy Storage via Gradient-Laminated Ceramifiable Silicone Foams"],"prefix":"10.1007","volume":"18","author":[{"given":"Shuilai","family":"Qiu","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingyao","family":"Xu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Congling","family":"Shi","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Laibin","family":"Zhang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,5,24]]},"reference":[{"key":"2228_CR1","doi-asserted-by":"publisher","first-page":"100390","DOI":"10.1016\/j.etran.2024.100390","volume":"24","author":"Z Jia","year":"2025","unstructured":"Z. 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