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Distinct from strategies employing pre-formed polymers, this work proposes an innovative monomer-induced in situ interface engineering strategy. By leveraging the preferential adsorption of acrylamide monomers on the Zn surface, a locally high-concentration region is created, which subsequently enables the in situ construction of a stable hydrated network interphase (HNI) triggered synergistically by Zn\n                    <jats:sup>2+<\/jats:sup>\n                    and SO\n                    <jats:sub>4<\/jats:sub>\n                    <jats:sup>2\u2212<\/jats:sup>\n                    during electrochemical cycling. The HNI precisely regulates Zn deposition via a triple synergistic mechanism: Lewis acid\u2013base coordination (C\u2009=\u2009O\u00b7\u00b7\u00b7Zn\n                    <jats:sup>2+<\/jats:sup>\n                    ) provides fixed nucleation sites; dynamically anchored SO\n                    <jats:sub>4<\/jats:sub>\n                    <jats:sup>2\u2212<\/jats:sup>\n                    within the interphase forms negatively charged microregions that homogenize Zn\n                    <jats:sup>2+<\/jats:sup>\n                    flux via Coulombic repulsion; and a dense hydrogen-bonding network effectively confines free water and suppresses side reactions. Benefiting from this multifunctional interphase, the Zn\/\/Zn symmetric cell achieves an ultra-long cycling life of 8650 h (over 360\u00a0days) at 1\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    with excellent reproducibility, the Zn\/\/Ti cell delivers a high average Coulombic efficiency of 99.71% at 5\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . The Zn\/\/I\n                    <jats:sub>2<\/jats:sub>\n                    full cell retains 89.15% of its capacity after 12,000 cycles. This work provides a novel paradigm for interfacial construction toward high-performance zinc metal anodes.\n                  <\/jats:p>","DOI":"10.1007\/s40820-026-02262-0","type":"journal-article","created":{"date-parts":[[2026,6,29]],"date-time":"2026-06-29T03:52:57Z","timestamp":1782705177000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Hydrated Network Interphase with Dynamic Negatively Charged Microregion Enables Ultra-Stable Aqueous Zinc-Ion Batteries"],"prefix":"10.1007","volume":"18","author":[{"given":"Yin","family":"Yang","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaofang","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xin","family":"Chen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jia","family":"Yao","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Daigan","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Luyang","family":"Ge","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fei","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lin","family":"Lv","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Li","family":"Tao","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hao","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Houzhao","family":"Wan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,6,29]]},"reference":[{"issue":"6321","key":"2262_CR1","doi-asserted-by":"publisher","first-page":"126","DOI":"10.1126\/science.aam6284","volume":"355","author":"B Obama","year":"2017","unstructured":"B. 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