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Here, we introduce a fishing-net-inspired interfacial molecular network that imparts intrinsic durability through coordination chemistry and interfacial dipole engineering. The metal-anchored hierarchical network integrates transition metal nodes, rigid small-molecule frameworks, and dense amine-functionalized polymer sub-networks into a netlike architecture that enhances charge extraction while suppressing bidirectional ion migration. Devices incorporating this interlayer achieve power conversion efficiencies of 26.19% (1.53\u00a0eV), 24.11% (1.61\u00a0eV), and 20.00% (1.77\u00a0eV), with open-circuit voltages and fill factors all exceeding 90% of the Shockley\u2013Queisser radiative limit. Notably, this performance is maintained even in wide-bandgap flexible devices. Flexible perovskite solar cells fabricated entirely under ambient air achieve 23.03% efficiency and retain 95% of their initial performance after 10,000 bending cycles. Moreover, the devices exhibit suppressed degradation during direct water immersion and reach a\n                    <jats:italic>T95<\/jats:italic>\n                    exceeding 2000\u00a0h under ambient conditions without encapsulation, establishing a broadly applicable interfacial design strategy for durable optoelectronics.\n                  <\/jats:p>","DOI":"10.1007\/s40820-026-02295-5","type":"journal-article","created":{"date-parts":[[2026,7,17]],"date-time":"2026-07-17T02:32:52Z","timestamp":1784255572000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Air-Processed and Water-Stable Perovskite Solar Cells Enabled by a Fishing-Net-Inspired Interfacial Network"],"prefix":"10.1007","volume":"18","author":[{"given":"Muh Fadhil","family":"Albab","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Muhammad","family":"Jahandar","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ah Ra","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinhee","family":"Heo","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yong Hyun","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Youngkyoo","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gi-Hwan","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ji-Youn","family":"Seo","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shinuk","family":"Cho","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Soyeon","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dong Chan","family":"Lim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,7,17]]},"reference":[{"issue":"6773","key":"2295_CR1","doi-asserted-by":"publisher","first-page":"638","DOI":"10.1126\/science.adw8780","volume":"390","author":"Z Xiong","year":"2025","unstructured":"Z. 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