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Here, we reveal that grain boundaries (GBs) in polycrystalline OCEs function as bipolar interfacial hotspots, accelerating three degradation pathways: lowering barriers for Li dendrite nucleation and enabling electron-leakage-driven reduction at anode side, while generating localized overpotentials for cathode phase transformation. To deactivate these GB-driven hotspots, we develop a laser-induced amorphization strategy that constructs a GB-free amorphous interlayer capable of homogenizing Li\n                    <jats:sup>+<\/jats:sup>\n                    flux and blocking electron migration. Applied to a representative sodium superionic conductor-type electrolyte, Li\n                    <jats:sub>1.3<\/jats:sub>\n                    Al\n                    <jats:sub>0.3<\/jats:sub>\n                    Ti\n                    <jats:sub>1.7<\/jats:sub>\n                    (PO\n                    <jats:sub>4<\/jats:sub>\n                    )\n                    <jats:sub>3<\/jats:sub>\n                    , this approach delivers substantially increased critical current density in Li symmetric cells (1.4 to 2.4\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    ) with stable cycling over 2000\u00a0h, and achieves an exceptional capacity retention of 101.9 mAh g\n                    <jats:sup>\u22121<\/jats:sup>\n                    after 800 cycles in LiCoO\n                    <jats:sub>2<\/jats:sub>\n                    full cells operated at 4.5\u00a0V. The generality of this strategy is further validated on garnet-type and perovskite-type OCEs. This work introduces amorphous interfacial current redistribution as a universal paradigm for engineering stable interfaces, providing a critical atomic-scale interface engineering route to unlock high-voltage, dendrite-free SSLMBs.\n                  <\/jats:p>","DOI":"10.1007\/s40820-026-02347-w","type":"journal-article","created":{"date-parts":[[2026,8,27]],"date-time":"2026-08-27T03:02:23Z","timestamp":1787799743000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Hotspot to Homogeneous: Amorphous Interfacial Current Redistribution Enables Stable Solid-State Lithium-Metal Batteries"],"prefix":"10.1007","volume":"19","author":[{"given":"Cuiyun","family":"Yang","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xupeng","family":"Lu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yexin","family":"Pan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qimeng","family":"Zhang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruohan","family":"Yu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rongliang","family":"Yang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huan","family":"Liu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Molong","family":"Duan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mitch Guijun","family":"Li","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyi","family":"Zhu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenghao","family":"Yang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,8,27]]},"reference":[{"issue":"3","key":"2347_CR1","doi-asserted-by":"publisher","first-page":"230","DOI":"10.1038\/s41560-023-01208-9","volume":"8","author":"J Janek","year":"2023","unstructured":"J. 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