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However, LIG-MSC research and production has been centered on non-sustainable polymeric substrates, such as polyimide. In this work, it is presented a cost-effective, reproducible, and robust approach for the preparation of LIG structures via a one-step laser direct writing on chromatography paper. The developed strategy relies on soaking the paper in a 0.1\u00a0M sodium tetraborate solution (borax) prior to the laser processing. Borax acts as a fire-retardant agent, thus allowing the laser processing of sensitive substrates that other way would be easily destroyed under the high-energy beam. LIG on paper exhibiting low sheet resistance (30 \u03a9 sq<jats:sup>\u22121<\/jats:sup>) and improved electrode\/electrolyte interface was obtained by the proposed method. When used as microsupercapacitor electrodes, this laser-induced graphene resulted in specific capacitances of 4.6 mF cm<jats:sup>\u22122<\/jats:sup> (0.015\u00a0mA\u00a0cm<jats:sup>\u22122<\/jats:sup>). Furthermore, the devices exhibit excellent cycling stability (&gt;\u200910,000 cycles at 0.5\u00a0mA\u00a0cm<jats:sup>\u22122<\/jats:sup>) and good mechanical properties. By connecting the devices in series and parallel, it was also possible to control the voltage and energy delivered by the system. Thus, paper-based LIG-MSC can be used as energy storage devices for flexible, low-cost, and portable electronics. Additionally, due to their flexible design and architecture, they can be easily adapted to other circuits and applications with different power requirements.<\/jats:p>\n                <jats:p><jats:bold>Graphical Abstract<\/jats:bold><\/jats:p>","DOI":"10.1007\/s00604-022-05610-0","type":"journal-article","created":{"date-parts":[[2022,12,30]],"date-time":"2022-12-30T23:02:36Z","timestamp":1672441356000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":89,"title":["Paper-based laser-induced graphene for sustainable and flexible microsupercapacitor applications"],"prefix":"10.1007","volume":"190","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4217-3842","authenticated-orcid":false,"given":"Jo\u00e3o","family":"Coelho","sequence":"first","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9285-3569","authenticated-orcid":false,"given":"Ricardo F.","family":"Correia","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3560-4317","authenticated-orcid":false,"given":"Sara","family":"Silvestre","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8346-4198","authenticated-orcid":false,"given":"Tom\u00e1s","family":"Pinheiro","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6878-1040","authenticated-orcid":false,"given":"Ana C.","family":"Marques","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3781-0085","authenticated-orcid":false,"given":"M. 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