{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,7,2]],"date-time":"2026-07-02T17:02:03Z","timestamp":1783011723224,"version":"3.54.6"},"reference-count":50,"publisher":"Elsevier BV","license":[{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"tdm","delay-in-days":0,"URL":"https:\/\/www.elsevier.com\/tdm\/userlicense\/1.0\/"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"tdm","delay-in-days":0,"URL":"https:\/\/www.elsevier.com\/legal\/tdmrep-license"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-017"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-012"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2025,3,1]],"date-time":"2025-03-01T00:00:00Z","timestamp":1740787200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-004"}],"funder":[{"DOI":"10.13039\/501100002860","name":"China Sponsorship Council","doi-asserted-by":"publisher","id":[{"id":"10.13039\/501100002860","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100012774","name":"Innovationsfonden","doi-asserted-by":"publisher","id":[{"id":"10.13039\/100012774","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100004543","name":"China Scholarship Council","doi-asserted-by":"publisher","award":["9067-0040B"],"award-info":[{"award-number":["9067-0040B"]}],"id":[{"id":"10.13039\/501100004543","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["elsevier.com","sciencedirect.com"],"crossmark-restriction":true},"short-container-title":["Environmental Pollution"],"published-print":{"date-parts":[[2025,3]]},"DOI":"10.1016\/j.envpol.2024.125578","type":"journal-article","created":{"date-parts":[[2025,1,14]],"date-time":"2025-01-14T00:14:06Z","timestamp":1736813646000},"page":"125578","update-policy":"https:\/\/doi.org\/10.1016\/elsevier_cm_policy","source":"Crossref","is-referenced-by-count":25,"special_numbering":"C","title":["Nitrogen doping turns carbonaceous materials into fast-reacting catalysts for reductive dechlorination"],"prefix":"10.1016","volume":"368","author":[{"given":"Hui","family":"Ma","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8617-2393","authenticated-orcid":false,"given":"Hans Christian B.","family":"Hansen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shengyan","family":"Pu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7076-6894","authenticated-orcid":false,"given":"Qiong","family":"Ouyang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lisbeth Garbrecht","family":"Thygesen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dominique J.","family":"Tobler","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"78","reference":[{"key":"10.1016\/j.envpol.2024.125578_bib1","doi-asserted-by":"crossref","DOI":"10.1016\/j.cej.2022.136770","article-title":"Fine-tuning green rust \u2212 bone char composite synthesis for efficient chlorinated ethylene remediation","volume":"446","author":"Ai","year":"2022","journal-title":"Chem. Eng. J."},{"key":"10.1016\/j.envpol.2024.125578_bib2","doi-asserted-by":"crossref","DOI":"10.1016\/j.jhazmat.2020.124724","article-title":"Biochar catalyzed dechlorination \u2013 which biochar properties matter?","volume":"406","author":"Ai","year":"2021","journal-title":"J. Hazard Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib3","doi-asserted-by":"crossref","first-page":"3643","DOI":"10.1021\/acs.est.9b07069","article-title":"Bone char mediated dechlorination of trichloroethylene by green rust","volume":"54","author":"Ai","year":"2020","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib4","first-page":"191","volume":"vol. 6","author":"Ai","year":"2019"},{"key":"10.1016\/j.envpol.2024.125578_bib5","doi-asserted-by":"crossref","first-page":"465","DOI":"10.1016\/j.carbon.2014.09.079","article-title":"A new nanoporous nitrogen-doped highly-efficient carbonaceous CO2 sorbent synthesized with inexpensive urea and petroleum coke","volume":"81","author":"Bai","year":"2015","journal-title":"Carbon"},{"key":"10.1016\/j.envpol.2024.125578_bib6","doi-asserted-by":"crossref","first-page":"26","DOI":"10.1021\/nn102598m","article-title":"Structural defects in graphene","volume":"5","author":"Banhart","year":"2011","journal-title":"ACS Nano"},{"key":"10.1016\/j.envpol.2024.125578_bib7","doi-asserted-by":"crossref","first-page":"1243","DOI":"10.1007\/s13762-017-1468-y","article-title":"A review on the synthesis and applications of green rust for environmental pollutant remediation","volume":"15","author":"Bhave","year":"2018","journal-title":"Int. J. Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib8","doi-asserted-by":"crossref","first-page":"636","DOI":"10.1016\/j.envpol.2016.06.025","article-title":"Evaluating the mobility of polymer-stabilised zero-valent iron nanoparticles and their potential to co-transport contaminants in intact soil cores","volume":"216","author":"Chekli","year":"2016","journal-title":"Environ. Pollut."},{"key":"10.1016\/j.envpol.2024.125578_bib9","doi-asserted-by":"crossref","first-page":"3436","DOI":"10.1021\/es8011047","article-title":"Identification of green rust in groundwater","volume":"43","author":"Christiansen","year":"2009","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib10","doi-asserted-by":"crossref","first-page":"4323","DOI":"10.1021\/es702196a","article-title":"Biotic and abiotic anaerobic transformations of trichloroethene and cis-1,2-dichloroethene in fractured sandstone","volume":"42","author":"Darlington","year":"2008","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib11","doi-asserted-by":"crossref","DOI":"10.1016\/j.watres.2022.119006","article-title":"N-doped biochar-catalyzed dechlorination of carbon tetrachloride in sulfide-containing aqueous solutions: performances, mechanisms and pathways","volume":"223","author":"Ding","year":"2022","journal-title":"Water Res."},{"key":"10.1016\/j.envpol.2024.125578_bib12","doi-asserted-by":"crossref","first-page":"14286","DOI":"10.1021\/acs.est.8b03565","article-title":"Nitrogen-doped carbon materials as metal-free catalyst for the dechlorination of trichloroethylene by sulfide","volume":"52","author":"Ding","year":"2018","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib13","article-title":"Pyrolysis of laurel (Laurus nobilis L.) extraction residues in a fixed-bed reactor: characterization of bio-oil and bio-char","volume":"88","author":"Erta\u015f","year":"2010"},{"key":"10.1016\/j.envpol.2024.125578_bib14","volume":"vol. 267","author":"Fu","year":"2014"},{"key":"10.1016\/j.envpol.2024.125578_bib15","doi-asserted-by":"crossref","first-page":"14284","DOI":"10.1021\/acscatal.1c03701","article-title":"Nature of intrinsic defects in carbon materials for electrochemical dechlorination of 1, 2-dichloroethane to ethylene","volume":"11","author":"Gan","year":"2021","journal-title":"ACS Catal."},{"key":"10.1016\/j.envpol.2024.125578_bib16","doi-asserted-by":"crossref","first-page":"10931","DOI":"10.1021\/acscatal.9b02853","article-title":"Identification of catalytic active sites in nitrogen-doped carbon for electrocatalytic dechlorination of 1,2-dichloroethane","volume":"9","author":"Gan","year":"2019","journal-title":"ACS Catal."},{"key":"10.1016\/j.envpol.2024.125578_bib17","doi-asserted-by":"crossref","first-page":"2284","DOI":"10.1021\/acsestengg.4c00241","article-title":"Unveiling the mechanistic role of surface nitrogen and sulfur in boosting the dechlorination performance of zero-valent iron","volume":"4","author":"Gong","year":"2024","journal-title":"ACS ES&T Eng."},{"key":"10.1016\/j.envpol.2024.125578_bib18","doi-asserted-by":"crossref","DOI":"10.1016\/j.jhazmat.2020.122620","article-title":"Effects of non-reducible dissolved solutes on reductive dechlorination of trichloroethylene by ball milled zero valent irons","volume":"396","author":"Gong","year":"2020","journal-title":"J. Hazard Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib19","doi-asserted-by":"crossref","first-page":"6317","DOI":"10.1021\/acs.est.8b00576","article-title":"Chlorate Formation mechanism in the presence of sulfate radical, chloride, bromide and natural organic matter","volume":"52","author":"Hou","year":"2018","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib20","doi-asserted-by":"crossref","first-page":"103","DOI":"10.1016\/j.jhazmat.2004.10.002","article-title":"Reactivity of Fe(II)\/cement systems in dechlorinating chlorinated ethylenes","volume":"118","author":"Hwang","year":"2005","journal-title":"J. Hazard Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib21","doi-asserted-by":"crossref","first-page":"9532","DOI":"10.1002\/adma.201602912","article-title":"Defect graphene as a trifunctional catalyst for electrochemical reactions","volume":"28","author":"Jia","year":"2016","journal-title":"Adv. Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib22","series-title":"Contaminants of Emerging Concern in Water and Wastewater","first-page":"299","article-title":"Chapter 9 - advanced oxidation processes for the treatment of contaminants of emerging concern","author":"Khan","year":"2020"},{"key":"10.1016\/j.envpol.2024.125578_bib23","doi-asserted-by":"crossref","first-page":"4693","DOI":"10.1021\/ef200915s","article-title":"Surface functionality and carbon structures in lignocellulosic-derived biochars produced by fast pyrolysis","volume":"25","author":"Kim","year":"2011","journal-title":"Energy Fuel."},{"key":"10.1016\/j.envpol.2024.125578_bib24","series-title":"Recent Advances in Pyrolysis","article-title":"Influence of process parameters on synthesis of biochar by pyrolysis of biomass: an alternative source of energy","author":"Krishna","year":"2019"},{"key":"10.1016\/j.envpol.2024.125578_bib25","doi-asserted-by":"crossref","DOI":"10.1016\/j.scitotenv.2022.153825","article-title":"Pyridinic nitrogen enables dechlorination of trichloroethylene to acetylene by green rust: performance, mechanism and applications","volume":"824","author":"Li","year":"2022","journal-title":"Sci. Total Environ."},{"key":"10.1016\/j.envpol.2024.125578_bib26","doi-asserted-by":"crossref","first-page":"312","DOI":"10.1016\/j.apcatb.2019.05.014","article-title":"From rice straw to magnetically recoverable nitrogen doped biochar: efficient activation of peroxymonosulfate for the degradation of metolachlor","volume":"254","author":"Liu","year":"2019","journal-title":"Appl. Catal. B Environ."},{"key":"10.1016\/j.envpol.2024.125578_bib27","doi-asserted-by":"crossref","DOI":"10.1016\/j.envpol.2021.116915","article-title":"Hexachloroethane dechlorination in sulfide-containing aqueous solutions catalyzed by nitrogen-doped carbon materials","volume":"281","author":"Liu","year":"2021","journal-title":"Environ. Pollut."},{"key":"10.1016\/j.envpol.2024.125578_bib28","doi-asserted-by":"crossref","DOI":"10.1016\/j.cej.2020.124015","article-title":"Urea-assisted one-step fabrication of a novel nitrogen-doped carbon fiber aerogel from cotton as metal-free catalyst in peroxymonosulfate activation for efficient degradation of carbamazepine","volume":"386","author":"Liu","year":"2020","journal-title":"Chem. Eng. J."},{"key":"10.1016\/j.envpol.2024.125578_bib29","doi-asserted-by":"crossref","DOI":"10.1016\/j.watres.2023.120999","article-title":"Persistent free radicals on biochar for its catalytic capability: a review","volume":"250","author":"Liu","year":"2024","journal-title":"Water Res."},{"key":"10.1016\/j.envpol.2024.125578_bib30","doi-asserted-by":"crossref","DOI":"10.1016\/j.cej.2021.132496","article-title":"Element doping of biochars enhances catalysis of trichloroethylene dechlorination","volume":"428","author":"Ma","year":"2022","journal-title":"Chem. Eng. J."},{"key":"10.1016\/j.envpol.2024.125578_bib31","article-title":"Electrocatalytic dechlorination of chloroethylenes using nitrogen-doped graphene electrodes","volume":"156947","author":"Ma","year":"2024","journal-title":"Chem. Eng. J."},{"key":"10.1016\/j.envpol.2024.125578_bib32","doi-asserted-by":"crossref","first-page":"4389","DOI":"10.1021\/acs.est.8b06480","article-title":"The structure of sulfidized zero-valent iron by one-pot synthesis: impact on contaminant selectivity and long-term performance","volume":"53","author":"Mangayayam","year":"2019","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib33","first-page":"173","volume":"vol. 146","author":"Mangayayam","year":"2018"},{"key":"10.1016\/j.envpol.2024.125578_bib34","doi-asserted-by":"crossref","first-page":"1852","DOI":"10.1016\/S0043-1354(02)00564-X","article-title":"Activated carbon adsorption of trichloroethylene (TCE) vapor stripped from TCE-contaminated water","volume":"37","author":"Miyake","year":"2003","journal-title":"Water Res."},{"key":"10.1016\/j.envpol.2024.125578_bib35","doi-asserted-by":"crossref","DOI":"10.1016\/j.jhazmat.2023.132772","article-title":"Field demonstration of in-situ microemulsion flushing for enhanced remediation of multiple chlorinated solvents contaminated aquifer","volume":"463","author":"Mo","year":"2024","journal-title":"J. Hazard Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib36","doi-asserted-by":"crossref","first-page":"4167","DOI":"10.1021\/acs.est.2c06433","article-title":"Decoupling Fe0 application and bioaugmentation in space and time enables microbial reductive dechlorination of trichloroethene to ethene: evidence from soil columns","volume":"57","author":"Mohana Rangan","year":"2023","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib37","volume":"vol. 244","author":"Ouyang","year":"2023"},{"key":"10.1016\/j.envpol.2024.125578_bib38","doi-asserted-by":"crossref","first-page":"15996","DOI":"10.1016\/j.ijhydene.2014.01.045","article-title":"Exploring the active sites of nitrogen-doped graphene as catalysts for the oxygen reduction reaction","volume":"39","author":"Ouyang","year":"2014","journal-title":"Int. J. Hydrogen Energy"},{"key":"10.1016\/j.envpol.2024.125578_bib39","first-page":"955","volume":"vol. 12","author":"Rado\u0144","year":"2017"},{"key":"10.1016\/j.envpol.2024.125578_bib40","doi-asserted-by":"crossref","first-page":"40","DOI":"10.1016\/j.apsusc.2016.11.181","article-title":"Significance of optimal N-doping in mesoporous carbon framework to achieve high specific capacitance","volume":"418","author":"Sahoo","year":"2017","journal-title":"Appl. Surf. Sci."},{"key":"10.1016\/j.envpol.2024.125578_bib41","doi-asserted-by":"crossref","first-page":"101","DOI":"10.3109\/07388551.2012.727080","article-title":"Current trends in trichloroethylene biodegradation: a review","volume":"34","author":"Shukla","year":"2014","journal-title":"Crit. Rev. Biotechnol."},{"key":"10.1016\/j.envpol.2024.125578_bib42","doi-asserted-by":"crossref","DOI":"10.1016\/j.jhazmat.2022.130315","article-title":"Selective dechlorination degradation of chlorobenzenes by dual single-atomic Fe\/Ni catalyst with M-N\/M-O active sites synergistic","volume":"443","author":"Tang","year":"2023","journal-title":"J. Hazard Mater."},{"key":"10.1016\/j.envpol.2024.125578_bib43","doi-asserted-by":"crossref","DOI":"10.1016\/j.apcatb.2023.122852","article-title":"Insights into molecular imprinting polydopamine in-situ activating peroxydisulfate for targeted removal of refractory organic pollutants: overlooked N site","volume":"334","author":"Tang","year":"2023","journal-title":"Appl. Catal. B Environ."},{"key":"10.1016\/j.envpol.2024.125578_bib44","doi-asserted-by":"crossref","DOI":"10.1016\/j.watres.2023.120950","article-title":"Overlooked role of void-nanoconfined effect in emerging pollutant degradation: modulating the electronic structure of active sites to accelerate catalytic oxidation","volume":"249","author":"Tang","year":"2024","journal-title":"Water Res."},{"key":"10.1016\/j.envpol.2024.125578_bib45","doi-asserted-by":"crossref","DOI":"10.1016\/j.scitotenv.2021.151502","article-title":"Catalytic mechanism of nitrogen-doped biochar under different pyrolysis temperatures: the crucial roles of nitrogen incorporation and carbon configuration","volume":"816","author":"Wan","year":"2022","journal-title":"Sci. Total Environ."},{"key":"10.1016\/j.envpol.2024.125578_bib46","doi-asserted-by":"crossref","DOI":"10.1016\/j.cej.2020.126136","article-title":"Customised fabrication of nitrogen-doped biochar for environmental and energy applications","volume":"401","author":"Wan","year":"2020","journal-title":"Chem. Eng. J."},{"key":"10.1016\/j.envpol.2024.125578_bib47","volume":"vol. 291","author":"Xu","year":"2021"},{"key":"10.1016\/j.envpol.2024.125578_bib48","doi-asserted-by":"crossref","first-page":"2535","DOI":"10.1021\/es991279q","article-title":"Kinetics and mechanisms for TCE oxidation by permanganate","volume":"34","author":"Yan","year":"2000","journal-title":"Environ. Sci. Technol."},{"key":"10.1016\/j.envpol.2024.125578_bib49","doi-asserted-by":"crossref","first-page":"429","DOI":"10.1016\/j.jcis.2016.11.076","article-title":"Glycine buffered synthesis of layered iron(II)-iron(III) hydroxides (green rusts)","volume":"497","author":"Yin","year":"2017","journal-title":"J. Colloid Interface Sci."},{"key":"10.1016\/j.envpol.2024.125578_bib50","doi-asserted-by":"crossref","first-page":"7290","DOI":"10.1021\/acs.est.6b01897","article-title":"Environmental remediation and application of nanoscale zero-valent iron and its composites for the removal of heavy metal ions: a review","volume":"50","author":"Zou","year":"2016","journal-title":"Environ. Sci. Technol."}],"container-title":["Environmental Pollution"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/api.elsevier.com\/content\/article\/PII:S0269749124022954?httpAccept=text\/xml","content-type":"text\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/api.elsevier.com\/content\/article\/PII:S0269749124022954?httpAccept=text\/plain","content-type":"text\/plain","content-version":"vor","intended-application":"text-mining"}],"deposited":{"date-parts":[[2025,4,16]],"date-time":"2025-04-16T20:46:10Z","timestamp":1744836370000},"score":1,"resource":{"primary":{"URL":"https:\/\/linkinghub.elsevier.com\/retrieve\/pii\/S0269749124022954"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2025,3]]},"references-count":50,"alternative-id":["S0269749124022954"],"URL":"https:\/\/doi.org\/10.1016\/j.envpol.2024.125578","relation":{},"ISSN":["0269-7491"],"issn-type":[{"value":"0269-7491","type":"print"}],"subject":[],"published":{"date-parts":[[2025,3]]},"assertion":[{"value":"Elsevier","name":"publisher","label":"This article is maintained by"},{"value":"Nitrogen doping turns carbonaceous materials into fast-reacting catalysts for reductive dechlorination","name":"articletitle","label":"Article Title"},{"value":"Environmental Pollution","name":"journaltitle","label":"Journal Title"},{"value":"https:\/\/doi.org\/10.1016\/j.envpol.2024.125578","name":"articlelink","label":"CrossRef DOI link to publisher maintained version"},{"value":"article","name":"content_type","label":"Content Type"},{"value":"\u00a9 2025 Elsevier Ltd. All rights are reserved, including those for text and data mining, AI training, and similar technologies.","name":"copyright","label":"Copyright"}],"article-number":"125578"}}