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Solution casting, slow air drying, hot pressing, and reinforcement by cellulose nanocrystals afforded films (\u223c100 \u03bcm thickness) that feature intriguing properties: they have very smooth surfaces (SEM), are highly flexible, and have good light transmittance for both the visible and near-infrared range (89\u201391%), high tensile strength (81\u2013122 MPa), and modulus of elasticity (3.4\u20134.0 GPa) depending on hydration state and respective water content. The extraordinarily low oxygen permeation of &amp;lt;0.005 cm3 \u03bcm m\u20132 day\u20131 kPa\u20131 (50% RH) and &amp;lt;0.03 cm3 \u03bcm m\u20132 day\u20131 kPa\u20131 (80% RH) can be regarded as a particularly interesting feature of DAC films. The unusually high initial contact angle of about 67\u00b0 revealed a rather low hydrophilicity compared to other oxidatively modified or unmodified cellulosic materials which is most likely the result of inter- and intramolecular hemiacetal and hemialdal formation during drying and pressing.<\/jats:p>","DOI":"10.1021\/acs.biomac.8b00536","type":"journal-article","created":{"date-parts":[[2018,5,14]],"date-time":"2018-05-14T15:28:46Z","timestamp":1526311726000},"page":"2969-2978","source":"Crossref","is-referenced-by-count":176,"title":["Transparent, Flexible, and Strong 2,3-Dialdehyde Cellulose\nFilms with High Oxygen Barrier Properties"],"prefix":"10.1021","volume":"19","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3210-3859","authenticated-orcid":true,"given":"Sven F.","family":"Plappert","sequence":"first","affiliation":[{"name":"University of Natural Resources and Life Sciences Vienna , , Konrad-Lorenz-Stra\u00dfe 24 , ,","place":["Tulln, Austria, A-3430"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sakeena","family":"Quraishi","sequence":"additional","affiliation":[{"name":"University of Natural Resources and Life Sciences Vienna , , Konrad-Lorenz-Stra\u00dfe 24 , ,","place":["Tulln, Austria, A-3430"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nicole","family":"Pircher","sequence":"additional","affiliation":[{"name":"University of Natural Resources and Life Sciences Vienna , , Konrad-Lorenz-Stra\u00dfe 24 , ,","place":["Tulln, Austria, A-3430"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kirsi S.","family":"Mikkonen","sequence":"additional","affiliation":[{"name":"University of Helsinki , , P.O. 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