{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,11]],"date-time":"2026-10-11T03:43:09Z","timestamp":1791690189655,"version":"4.3.4"},"reference-count":77,"publisher":"American Chemical Society (ACS)","issue":"12","license":[{"start":{"date-parts":[[2015,6,1]],"date-time":"2015-06-01T00:00:00Z","timestamp":1433116800000},"content-version":"vor","delay-in-days":26,"URL":"https:\/\/pubs.acs.org\/page\/policy\/authorchoice_termsofuse.html"}],"funder":[{"DOI":"10.13039\/100006151","name":"Basic Energy Sciences","doi-asserted-by":"publisher","award":["NA"],"award-info":[{"award-number":["NA"]}],"id":[{"id":"10.13039\/100006151","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2015,6,16]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>In geologic carbon sequestration, capillary pressure (Pc)\u2013saturation (Sw) relations are needed to predict reservoir processes. Capillarity and its hysteresis have been extensively studied in oil\u2013water and gas\u2013water systems, but few measurements have been reported for supercritical (sc) CO2\u2013water. Here, Pc\u2013Sw relations of scCO2 displacing brine (drainage), and brine rewetting (imbibition) were studied to understand CO2 transport and trapping behavior under reservoir conditions. Hysteretic drainage and imbibition Pc\u2013Sw curves were measured in limestone sands at 45 \u00b0C under elevated pressures (8.5 and 12.0 MPa) for scCO2\u2013brine, and in limestone and dolomite sands at 23 \u00b0C (0.1 MPa) for air\u2013brine using a new computer programmed porous plate apparatus. scCO2\u2013brine drainage and imbibition curves shifted to lower Pc relative to predictions based on interfacial tension, and therefore deviated from capillary scaling predictions for hydrophilic interactions. Fitting universal scaled drainage and imbibition curves show that wettability alteration resulted from scCO2 exposure over the course of months-long experiments. Residual trapping of the nonwetting phases was determined at Pc = 0 during imbibition. Amounts of trapped scCO2 were significantly larger than for those for air, and increased with pressure (depth), initial scCO2 saturation, and time. These results have important implications for scCO2 distribution, trapping, and leakage potential.<\/jats:p>","DOI":"10.1021\/acs.est.5b00826","type":"journal-article","created":{"date-parts":[[2015,5,6]],"date-time":"2015-05-06T13:27:37Z","timestamp":1430918857000},"page":"7208-7217","source":"Crossref","is-referenced-by-count":99,"title":["Capillary\nPressure\u2013Saturation Relations for\nSupercritical CO2 and Brine in Limestone\/Dolomite Sands:\nImplications for Geologic Carbon Sequestration in Carbonate Reservoirs"],"prefix":"10.1021","volume":"49","author":[{"given":"Shibo","family":"Wang","sequence":"first","affiliation":[{"name":"Lawrence Berkeley National Laboratory , , 1 Cyclotron Road , , ,","place":["Berkeley, California, United States, 94720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tetsu K.","family":"Tokunaga","sequence":"additional","affiliation":[{"name":"Lawrence Berkeley National Laboratory , , 1 Cyclotron Road , , ,","place":["Berkeley, California, United States, 94720"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2015,5,6]]},"reference":[{"key":"2026090120303142300_cit1","first-page":"195","volume-title":"Underground Geological\nStorage, in IPCC Special Report on Carbon Dioxide Capture and Storage","author":"Intergovernmental Panel on Climate Change (IPCC).","year":"2005"},{"key":"2026090120303142300_cit2","doi-asserted-by":"crossref","first-page":"52","DOI":"10.2118\/05-10-05","article-title":"Geomechanical\nfactors affecting geological\nstorage of CO2 in depleted oil and gas reservoirs","volume":"44","author":"Hawkes","year":"2005","journal-title":"J. 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