{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,11]],"date-time":"2026-08-11T16:25:04Z","timestamp":1786465504304,"version":"build-2736575974"},"reference-count":113,"publisher":"American Chemical Society (ACS)","issue":"31","license":[{"start":{"date-parts":[[2026,7,27]],"date-time":"2026-07-27T00:00:00Z","timestamp":1785110400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,7,27]],"date-time":"2026-07-27T00:00:00Z","timestamp":1785110400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,7,27]],"date-time":"2026-07-27T00:00:00Z","timestamp":1785110400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22306059"],"award-info":[{"award-number":["22306059"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["531118010830"],"award-info":[{"award-number":["531118010830"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/na","name":"Science and Technology Innovation Program of Guangdong Province","doi-asserted-by":"publisher","award":["2024A1515011937"],"award-info":[{"award-number":["2024A1515011937"]}],"id":[{"id":"10.13039\/na","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/na","name":"Science and Technology Innovation Program of Hunan Province","doi-asserted-by":"publisher","award":["2024RC3106"],"award-info":[{"award-number":["2024RC3106"]}],"id":[{"id":"10.13039\/na","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/na","name":"Science and Technology Innovation Program of Hunan Province","doi-asserted-by":"publisher","award":["2025AQ2001"],"award-info":[{"award-number":["2025AQ2001"]}],"id":[{"id":"10.13039\/na","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/na","name":"State Key Laboratory of Advanced Environmental Technology","doi-asserted-by":"publisher","award":["SKLAET202512"],"award-info":[{"award-number":["SKLAET202512"]}],"id":[{"id":"10.13039\/na","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,11]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Highly functionalized particle-phase organic nitrates (ONs) contribute substantially to secondary organic aerosol and influence NOx cycling through multiphase transformations. While photolysis of particle-phase inorganic nitrates is known to release nitrous acid to influence atmospheric oxidation, particle-phase ON photolysis remains poorly constrained. In this study, we determine suspended particle-phase photolysis rate constants for five synthetic multifunctional ONs and sulfur-substituted ONs (SONs) under dry conditions, using an oxidation flow reactor coupled to online aerosol measurements. The compounds include limonene- (LmSON, LmON), styrene- (SySON, SyON), and \u03b2-caryophyllene-derived (BcyON) species with additional carbonyl, sulfate, aromatic, or hydroxyl functionalities. We measure absorption cross-sections, infer quantum yields, and extrapolate to ambient solar conditions. The ambient particle-phase lifetimes range from 5.7 to 1.4 h, whereas no detectable photolysis for BcyON. Notably, carbonyl\u2013nitrooxy conjugation enhances absorption at atmospherically relevant wavelengths and yields the fastest photolysis. We also observe net NOx production during photolysis, demonstrating its potential to influence NOx recycling. These results identify photolysis as an important sink for particle-phase ONs under dry conditions, with measurable effects on reactive nitrogen budgets. Given the functionalization typical of ambient ONs, particle-phase photolysis may be relatively rapid, highlighting the need to incorporate this pathway and its mechanistic controls into atmospheric models.<\/jats:p>","DOI":"10.1021\/acs.est.6c00126","type":"journal-article","created":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T13:11:27Z","timestamp":1785849087000},"page":"21766-21778","source":"Crossref","is-referenced-by-count":0,"title":["Particle-Phase Photolysis\nof Organic Nitrates and\nSulfur-Substituted Organic Nitrates: Constraints on Atmospheric Lifetimes\nand Loss Pathways"],"prefix":"10.1021","volume":"60","author":[{"given":"Xiang","family":"Zhang","sequence":"first","affiliation":[{"name":"Hunan University , , , ,","place":["Changsha, Hunan, China, 410082"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2941-7235","authenticated-orcid":true,"given":"Yuchen","family":"Wang","sequence":"additional","affiliation":[{"name":"Hunan University , , , ,","place":["Changsha, Hunan, China, 410082"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhijun","family":"Yang","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mingkai","family":"Liu","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8512-0663","authenticated-orcid":true,"given":"Wei","family":"Song","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-3732-2291","authenticated-orcid":true,"given":"Xiangyu","family":"Zhang","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruicheng","family":"Zhou","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tianli","family":"Xiong","sequence":"additional","affiliation":[{"name":"Hunan University , , , ,","place":["Changsha, Hunan, China, 410082"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3041-0329","authenticated-orcid":true,"given":"Bin","family":"Yuan","sequence":"additional","affiliation":[{"name":"Jinan University , , ,","place":["Guangzhou, China, 511443"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3031-701X","authenticated-orcid":true,"given":"Andrew T.","family":"Lambe","sequence":"additional","affiliation":[{"name":"Aerodyne Research Inc. , , ,","place":["Billerica, Massachusetts, United States, 01821"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weiwei","family":"Hu","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1982-0928","authenticated-orcid":true,"given":"Xinming","family":"Wang","sequence":"additional","affiliation":[{"name":"Guangzhou Institute of Geochemistry, Chinese Academy of Sciences , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,27]]},"reference":[{"issue":"9","key":"2026081110082603700_cit1","doi-asserted-by":"publisher","first-page":"5421","DOI":"10.1021\/acs.est.1c08380","article-title":"Partitioning\nof Organonitrates in the Production of Secondary Organic Aerosols\nfrom \u03b1-Pinene Photo-Oxidation","volume":"56","author":"Aruffo","year":"2022","journal-title":"Environ.\nSci. 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Total Environ."},{"issue":"4","key":"2026081110082603700_cit20","doi-asserted-by":"publisher","first-page":"2351","DOI":"10.5194\/acp-22-2351-2022","article-title":"Enhanced Summertime\nOzone and SOA from Biogenic Volatile Organic Compound (BVOC) Emissions\nDue to Vegetation Biomass Variability during 1981\u20132018 in China","volume":"22","author":"Cao","year":"2022","journal-title":"Atmos. Chem. Phys."},{"issue":"23","key":"2026081110082603700_cit21","doi-asserted-by":"publisher","first-page":"13738","DOI":"10.1021\/acs.est.8b03861","article-title":"Constraints on Aerosol\nNitrate Photolysis as a Potential Source of HONO and NOx","volume":"52","author":"Romer","year":"2018","journal-title":"Environ. Sci. 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Model Dev."},{"issue":"4","key":"2026081110082603700_cit27","doi-asserted-by":"publisher","first-page":"1703","DOI":"10.5194\/gmd-10-1703-2017","article-title":"Description and Evaluation of the\nCommunity Multiscale Air Quality (CMAQ) Modeling System Version 5.1","volume":"10","author":"Appel","year":"2017","journal-title":"Geosci. Model. Dev."},{"issue":"6","key":"2026081110082603700_cit28","doi-asserted-by":"publisher","first-page":"1516","DOI":"10.1073\/pnas.1508108113","article-title":"Highly Functionalized Organic Nitrates\nin the Southeast United States: Contribution to Secondary Organic\nAerosol and Reactive Nitrogen Budgets","volume":"113","author":"Lee","year":"2016","journal-title":"Proc.\nNatl. Acad. Sci. U. S. 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Environ."},{"issue":"9","key":"2026081110082603700_cit35","doi-asserted-by":"publisher","first-page":"3516","DOI":"10.1073\/pnas.1006461108","article-title":"Identifying Organic Aerosol Sources\nby Comparing Functional Group Composition in Chamber and Atmospheric\nParticles","volume":"108","author":"Russell","year":"2011","journal-title":"Proc. Natl. Acad. Sci. U. S. A."},{"issue":"9","key":"2026081110082603700_cit36","doi-asserted-by":"publisher","first-page":"4543","DOI":"10.5194\/acp-13-4543-2013","article-title":"Observations of Total RONO2 over the Boreal Forest:\nNOx Sinks and HNO3 Sources","volume":"13","author":"Browne","year":"2013","journal-title":"Atmos. Chem. Phys."},{"issue":"5","key":"2026081110082603700_cit37","doi-asserted-by":"publisher","DOI":"10.1073\/pnas.1418702112","article-title":"Rapid Deposition\nof Oxidized Biogenic Compounds to a Temperate Forest","volume":"112","author":"Nguyen","year":"2015","journal-title":"Proc. Natl. Acad. Sci. U. S. 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Chem."},{"issue":"5","key":"2026081110082603700_cit41","doi-asserted-by":"publisher","first-page":"2878","DOI":"10.1021\/acs.est.0c06838","article-title":"Optical Properties\nof Secondary Organic\nAerosol Produced by Nitrate Radical Oxidation of Biogenic Volatile\nOrganic Compounds","volume":"55","author":"He","year":"2021","journal-title":"Environ. Sci. Technol."},{"issue":"10","key":"2026081110082603700_cit42","doi-asserted-by":"publisher","first-page":"5851","DOI":"10.5194\/acp-23-5851-2023","article-title":"On the Importance of Multiphase Photolysis of Organic Nitrates on\nTheir Global Atmospheric Removal","volume":"23","author":"Gonza\u0301lez-Sa\u0301nchez","year":"2023","journal-title":"Atmos. 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